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Mechanisms Controlling Soot Formation In Diffusion Flames
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Book Synopsis Mechanisms Controlling Soot Formation in Diffusion Flames by :
Download or read book Mechanisms Controlling Soot Formation in Diffusion Flames written by and published by . This book was released on 1997 with total page 94 pages. Available in PDF, EPUB and Kindle. Book excerpt: Arclength continuation methods were incorporated into a code for predicting the structure of sooting, opposed-jet flames. The code includes complex chemistry, detailed particle dynamics, particle chemistry and radiation. The code was used to predict soot production over a wide variation in strain rates for both ethylene/air and methane/air diffusion flames. Predicted values (both peak and spatial distributions) agree well with experimental measurements in ethylene flames. Particle size distributions are also predicted using the aerosol equations from MAEROS, but no data is available for comparison. Also, the soot dynamical equations were imbedded into a separate code to describe soot production in a coflow, laminar, diffusion flame which includes treatment of detailed, gas phase chemistry. Predictions were compared to measurements made in a methane, coflow flame. Reasonable agreement between the predictions and measurements was obtained, although a factor of three underprediction of the soot volume fractions is likely due to uncertainties in inlet conditions and an inability to match closely bulk flame parameters such as temperature. Predicted peak soot production occurred around 1720K and particle oxidation was dominated by superequilibrium concentrations of hydroxyl radicals. Several PAH-forming sequences were examined and compared to the traditional acetylene-addition sequence. A sequence involving benzyl-propargyl combination was found to compete with the traditional mechanism and it should be included in future analyses. The algorithms for treating sectional soot dynamics and growth/oxidation rates were modified to include effects at high pressure. Continuum effects and limitations to gaseous diffusion were included in the opposed jet code. Predicted variations in soot production due to pressure changes from 4 to 10 atmospheres were made for an ethylene-air.
Book Synopsis Soot Formation in Combustion by : Henning Bockhorn
Download or read book Soot Formation in Combustion written by Henning Bockhorn and published by Springer Science & Business Media. This book was released on 2013-03-08 with total page 595 pages. Available in PDF, EPUB and Kindle. Book excerpt: Soot Formation in Combustion represents an up-to-date overview. The contributions trace back to the 1991 Heidelberg symposium entitled "Mechanism and Models of Soot Formation" and have all been reedited by Prof. Bockhorn in close contact with the original authors. The book gives an easy introduction to the field for newcomers, and provides detailed treatments for the specialists. The following list of contents illustrates the topics under review:
Book Synopsis Fundamental Mechanisms for CO and Soot Formation in Diffusion Flames. Annual Progress Report and Quarterly Report. April 1, 1992-August 31, 1992 by : R. J. Santoro
Download or read book Fundamental Mechanisms for CO and Soot Formation in Diffusion Flames. Annual Progress Report and Quarterly Report. April 1, 1992-August 31, 1992 written by R. J. Santoro and published by . This book was released on 1993 with total page pages. Available in PDF, EPUB and Kindle. Book excerpt:
Book Synopsis Soot in Combustion Systems and Its Toxic Properties by : J. Lahaye
Download or read book Soot in Combustion Systems and Its Toxic Properties written by J. Lahaye and published by Springer Science & Business Media. This book was released on 2013-04-17 with total page 429 pages. Available in PDF, EPUB and Kindle. Book excerpt: Our interest in Mulhouse for carbon black and soot began some 30 years ago when J.B. Donnet developed the concept of surface chemistry of carbon and its involvement in interactions with gas, liquid and solid phases. In the late sixties, we began to study soot formation in pyrolytic systems and later on in flames. The idea of organ1z1ng a meeting on soot formation originated some four or five years ago, through discussions among Professor J.B. Howard, Dr. A. D'Alessio and ourselves. At that time the scientific community was becoming aware of the necessity to strictly control soot formation and emission. Being involved in the study of surface properties of carbon black as well as of formation of soot, we realized that the combustion community was not always fully aware of the progress made by the physical-chemists on carbon black. Reciprocally, the carbon specialists were often ignoring the research carried out on soot in flames. One objective of this workshop was to stimulate discussions between these two scientific communities. During the preparation of the meeting, and especially during the review process by the Material Science Committee of the Scientific Affairs Division of N.A.T.O. the toxicological aspect emerged as being an important component to be addressed during the workshop. To reflect these preoccupations we invited biologists, physical chemists and engineers, all leaders in their field. The final programme is a compromise of the different aspects of the subject and was divided in five sessions.
Book Synopsis Effects of Pressure on the Mechanisms of Soot Formation and Oxidation in Laminar Diffusion Flames by : Chul Han Kim
Download or read book Effects of Pressure on the Mechanisms of Soot Formation and Oxidation in Laminar Diffusion Flames written by Chul Han Kim and published by . This book was released on 2005 with total page 408 pages. Available in PDF, EPUB and Kindle. Book excerpt:
Book Synopsis Soot Formation in Combustion by : Henning Bockhorn
Download or read book Soot Formation in Combustion written by Henning Bockhorn and published by . This book was released on 1995-01-01 with total page pages. Available in PDF, EPUB and Kindle. Book excerpt:
Book Synopsis Prediction of Soot Formation in Laminar Opposed Diffusion Flame with Detailed and Reduced Reaction Mechanisms by : Hojoon Chang
Download or read book Prediction of Soot Formation in Laminar Opposed Diffusion Flame with Detailed and Reduced Reaction Mechanisms written by Hojoon Chang and published by . This book was released on 2004 with total page pages. Available in PDF, EPUB and Kindle. Book excerpt: The present work focuses on a computational study of a simplified soot model to predict soot production and destruction in methane/oxidizer (O2 and N2) and ethylene/air flames using a one-dimensional laminar opposed diffusion flame setup. Two different detailed reaction mechanisms (361 reactions & 61 species for methane/oxidizer flame and 527 reactions & 99 species for ethylene/air flame) are used to validate the simplified soot model in each flame. The effects of strain rate and oxygen content on the soot production and destruction are studied, and the soot related properties such as soot volume fraction, particle number density and particle diameter are compared with published results. The results show reasonable agreement with data and that the soot volume fraction decreases with higher strain rate and lower oxygen content. The simplified soot model has also been used with two reduced reaction mechanisms (12-step, 16-species for methane flame and 20-species for ethylene flame) since such reduced mechanisms are computationally more efficient for practical application. The profiles of the physical properties and the major species are in excellent agreement with the results using the detailed reaction mechanisms. However, minor hydrocarbon-species such as acetylene (C2H2) that is the primary pyrolysis species in the simplified soot model is significantly over predicted and this, in turn, results in an over-prediction of soot production. Finally, the reduced reaction mechanism is modified to get more accurate prediction of the minor hydrocarbon-species. The modified reduced reaction mechanism shows that the soot prediction can be improved by improving the predictions of the key minor species.
Book Synopsis Hydrodynamic Effects on Soot Formation in Laminar Hydrocarbon-fueled Diffusion Flames by : Guozheng Lin
Download or read book Hydrodynamic Effects on Soot Formation in Laminar Hydrocarbon-fueled Diffusion Flames written by Guozheng Lin and published by . This book was released on 1996 with total page 568 pages. Available in PDF, EPUB and Kindle. Book excerpt:
Book Synopsis A Fundamental Study of Soot Formation in Diffusion Flames by : Richard L. Axelbaum
Download or read book A Fundamental Study of Soot Formation in Diffusion Flames written by Richard L. Axelbaum and published by . This book was released on 1988 with total page 510 pages. Available in PDF, EPUB and Kindle. Book excerpt:
Book Synopsis Particulate Carbon by : Donald Siegla
Download or read book Particulate Carbon written by Donald Siegla and published by Springer Science & Business Media. This book was released on 2013-11-11 with total page 500 pages. Available in PDF, EPUB and Kindle. Book excerpt: The goal of the symposium, "Particulate Carbon: Formation During Combustion", held at the General Motors Research Laboratories on October 15 and 16, 1980, was to discuss fundamental aspects of soot formation and oxidation in combustion systems and to stimulate new research by extensive interactions among the participants. This book contains lhe papers and discussions of that symposium, the 26th in an annual series covering many different disciplines which are timely and of interest to both General Motors and the technical community at large. The subject of this symposium has considerable relevance for man in his effort to control and preserve his environment. Emission of particulate carbon into the atmos phere from combustion sources is of concern to scientists and laymen alike. The hope of reducing this emission clearly requires an understanding of its formation during the combustion process, itself an area of considerable long-term research interest. It is our hope that this symposium has served to summarize what is known so that what remains to be learned can be pursued with greater vigor.
Book Synopsis Fuel Structure and Pressure Effects on the Formation of Soot Particles in Diffusion Flames by : Robert J. Santoro
Download or read book Fuel Structure and Pressure Effects on the Formation of Soot Particles in Diffusion Flames written by Robert J. Santoro and published by . This book was released on 1988 with total page 33 pages. Available in PDF, EPUB and Kindle. Book excerpt: During the first year of the present grant, efforts have concentrated on examining the effects of fuel molecular structure on soot formation in diffusion flames. Studies involving alkane, alkene, alkyne and aromatic fuel species have been studied with specific attention given to the surface growth process. Analysis of these studies has demonstrated a strong fuel structure dependence for the amount of soot formed, the conversion percentage of fuel carbon to soot, and the soot particle surface area present in these diffusion flames. However, when surface area taken into account, similar specific surface growth rate coefficients are observed for all the fuels studied. These results point to a similar surface growth process for all the fuels. Consistent with premixed flame results, the present studies show a continual decrease in this specific surface growth rate coefficient with time. Other effects of fuel structure observed include an acceleration of the inception of soot particles to lower locations and, thus, earlier times in the flame as soot conversion percentage increases. These results also point to the importance of the initial particle inception process which appears to control subsequent soot particle evolution. Keywords: Soot formation; Soot particles; Diffusion flames.
Book Synopsis Detailed Modeling of Soot Formation/oxidation in Laminar Coflow Diffusion Flames by : Qingan Zhang
Download or read book Detailed Modeling of Soot Formation/oxidation in Laminar Coflow Diffusion Flames written by Qingan Zhang and published by . This book was released on 2009 with total page 388 pages. Available in PDF, EPUB and Kindle. Book excerpt: The first goal of this thesis is to develop and validate a modeling tool into which fundamental combustion chemistry and aerosol dynamics theory are implemented for investigating soot formation/oxidation in multi-dimensional laminar coflow diffusion flames taking into account soot polydispersity and fractal-like aggregate structure. The second goal is to use the tool to study soot aggregate formation/oxidation in experimentally studied laminar coflow diffusion flames to advance the understanding of soot aggregate formation/oxidation mechanism.The first part of the thesis deals with the large CPU time problem when detailed models are coupled together. Using the domain decomposition method, a high performance parallel flame code is successfully developed. An advanced sectional aerosol dynamics model which can model fractal-like aggregate structure is successfully implemented into the parallel flame code. The performance of the parallel code is demonstrated through its application to the modeling of soot formation/oxidation in a laminar coflow CH4/air diffusion flame. The parallel efficiency reaches as high as 83%.In the third part of the thesis, the effects of oxidation-driven soot aggregate fragmentation on aggregate structure and soot oxidation rate are studied. Three fragmentation models with different fragmentation patterns are developed and implemented into the sectional aerosol dynamics model. The implementation of oxidation-driven aggregate fragmentation significantly improves the prediction of soot aggregate structure in the soot oxidation region.The second part of the thesis numerically explores soot aggregate formation in a laminar coflow C2H4/air diffusion flame using detailed PAH-based combustion chemistry and a PAH-based soot formation/oxidation model. Compared to the measured data, flame temperature, axial velocity, C2 H2 and OH concentrations, soot volume fraction, the average diameter and the number density of primary particles are reasonably well predicted. However, it is very challenging to predict effectively the average degree of particle aggregation. To do so, particle-particle and fluid-particle interactions that may cause non-unitary soot coagulation efficiency need to be considered. The original coagulation model is enhanced in this thesis to accommodate soot coagulation efficiency. Different types of soot coagulation efficiency are numerically investigated. It is found that a simple adjustment of soot coagulation efficiency from 100% to 20% provides good predictions on soot aggregate structure as well as flame properties.
Book Synopsis Soot Formation in Gaseous Laminar Diffusion Flames by : Changlie Wey
Download or read book Soot Formation in Gaseous Laminar Diffusion Flames written by Changlie Wey and published by . This book was released on 1984 with total page 386 pages. Available in PDF, EPUB and Kindle. Book excerpt:
Book Synopsis Soot Formation in Laminar Diffusion Flames by : eO L. Geulder
Download or read book Soot Formation in Laminar Diffusion Flames written by eO L. Geulder and published by . This book was released on 1989 with total page pages. Available in PDF, EPUB and Kindle. Book excerpt:
Book Synopsis Oxygen-Enhanced Combustion by : Charles E. Baukal Jr.
Download or read book Oxygen-Enhanced Combustion written by Charles E. Baukal Jr. and published by CRC Press. This book was released on 2013-03-15 with total page 779 pages. Available in PDF, EPUB and Kindle. Book excerpt: Combustion technology has traditionally been dominated by air/fuel combustion. However, two developments have increased the significance of oxygen-enhanced combustion-new technologies that produce oxygen less expensively and the increased importance of environmental regulations. Advantages of oxygen-enhanced combustion include less pollutant emissi
Book Synopsis The Second International Microgravity Combustion Workshop by :
Download or read book The Second International Microgravity Combustion Workshop written by and published by . This book was released on 1993 with total page 394 pages. Available in PDF, EPUB and Kindle. Book excerpt:
Book Synopsis ARO and AFOSR Contractors Meeting in Chemical Propulsion, Held in Virginia Beach, Virginia on 3-6 June 1996 by : David M. Mann
Download or read book ARO and AFOSR Contractors Meeting in Chemical Propulsion, Held in Virginia Beach, Virginia on 3-6 June 1996 written by David M. Mann and published by . This book was released on 1996 with total page 302 pages. Available in PDF, EPUB and Kindle. Book excerpt: Partial contents: Supercritical droplet behavior; Fundamentals of acoustic instabilities in liquid-propellant rockets; Modeling liquid jet atomization proceses; Liquid-propellant droplets dynamics and combustions in supercritical forced convective environments; Contributions of shear coaxial injectors to liquid rocket motor combustion instabilities; High pressure combustion studies under combustion driven oscillatory flow conditions; Droplet collision on liquid propellant combustion; Combustion and plumes; Development of a collisional radiative emission model for strongly nonequilibrium flows; Energy transfer processes in the production of excited states in reacting rocket flows; modeling nonequilibrium radiation in high altitude plumes; kinetics of plume radiation, and of HEDMs and metallic fuels combustion; Nonsteady combustion mechanisms of advanced solid propellants; Chemical mechanisms at the burning surface. p15
