Electronic Properties And Electron Electron Interaction Effects In Transition Metal Dichalcogenides

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Electronic Properties and Electron-electron Interaction Effects in Transition Metal Dichalcogenides

Author : Stefano Larentis
Publisher :
ISBN 13 :
Total Pages : 382 pages
Book Rating : 4.:/5 (15 download)

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Book Synopsis Electronic Properties and Electron-electron Interaction Effects in Transition Metal Dichalcogenides by : Stefano Larentis

Download or read book Electronic Properties and Electron-electron Interaction Effects in Transition Metal Dichalcogenides written by Stefano Larentis and published by . This book was released on 2018 with total page 382 pages. Available in PDF, EPUB and Kindle. Book excerpt: Transition metal dichalcogenides (TMDs) are a new class of two-dimensional layered materials characterized by a MX2 chemical formula, where M (X) stands for a transition metal (chalcogen). MoS2, MoSe2 and MoTe2 are semiconducting TMDs, which at the monolayer limit possess bandgaps >1 eV, rendering them attractive as possible channel material for scaled transistors. The bandstructures of monolayers feature coupled spin and valley degrees of freedom, thanks to large spin-orbit interaction, and large effective masses (m*), suggesting that electron-electron interaction effects are expected to be important in these semiconductors. In this dissertation we discuss the fabrication and electrical characterization of TMD-based electronic devices, with a focus on their electronic properties, including scattering mechanisms contributing to the mobility, carriers' effective mass, band offset in heterostructures, electronic compressibility, and spin susceptibility. We begin studying the four-point field-effect mobilities of few-layers MoS2, MoSe2 and MoTe2 field effect transistors (FETs), in top-contact, bottom-gate architectures. Using hexagonal boron-nitride dielectrics, we fabricate FETs with an improved bottom-contact, dual-gate architecture to probe transport at low temperatures in monolayer MoS2, and mono- and bilayer MoSe2. From conductivity and carrier density measurements we determine the Hall mobility, which shows strong temperature dependence, consistent with phonon scattering, and saturates at low temperatures because of impurity scattering. High mobility MoSe2 samples probed in perpendicular magnetic field, at low temperatures show Shubnikov-de Haas oscillations. Using magnetotransport we probe carriers in spin split bands at the K point in the conduction band and extract their m* = 0.8m [subscript e]; m [subscript e] is the bare electron mass. Quantum Hall states emerging at either odd or even filling factors are explained by a density dependent, interaction enhanced Zeeman splitting. Gated graphene-MoS2 heterostructures reveal a saturating electron branch conductivity at the onset of MoS2 population. Magnetotransport measurements probe the graphene electron density, which saturates and decreases as MoS2 populates, a finding associated with the negative compressibility of MoS2 electrons, modeled by a decreasing chemical potential, where many-body contributions dominate. Using a multi-gate architecture in monolayer MoTe2 FETs, that allows for independent contact resistance and threshold voltage tuning, we integrate reconfigurable n- and p-FETs, and demonstrate a complementary inverter.

Electron Spectroscopies Applied to Low-Dimensional Structures

Author : H.P. Hughes
Publisher : Springer Science & Business Media
ISBN 13 : 0306471264
Total Pages : 513 pages
Book Rating : 4.3/5 (64 download)

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Book Synopsis Electron Spectroscopies Applied to Low-Dimensional Structures by : H.P. Hughes

Download or read book Electron Spectroscopies Applied to Low-Dimensional Structures written by H.P. Hughes and published by Springer Science & Business Media. This book was released on 2006-04-11 with total page 513 pages. Available in PDF, EPUB and Kindle. Book excerpt: The effect of reduced dimensionality, inherent at the crystallographic level, on the electronic properties of low dimensional materials can be dramatic, leading to structural and electronic instabilities—including supercond- tivity at high temperatures, charge density waves, and localisation—which continue to attract widespread interest. The layered transition metal dichalcogenides have engaged attention for many years, partly arising from the charge density wave effects which some show and the controlled way in which their properties can be modified by intercalation, while the development of epitaxial growth techniques has opened up promising areas based on dichalcogenide heterostructures and quantum wells. The discovery of high-temperature superconducting oxides, and the realisation that polymeric materials too can be exploited in a controlled way for various opto-electronic applications, have further sti- lated interest in the effects of structural dimensionality. It seems timely therefore to draw together some strands of recent research involving a range of disparate materials which share some common char- teristics of low dimensionality. This resulting volume is aimed at researchers with specialist interests in the particular materials discussed but who may also wish to examine the related phenomena observed in different systems, and at a more general solid state audience with broad interests in electronic properties and low dimensional phenomena. Space limitations have required us to be selective as regards particular materials, though we have managed to include those as dissimilar as polymeric semiconductors, superconducting oxides, bronzes and layered chalcogenides.

Two Dimensional Transition Metal Dichalcogenides

Author : Narayanasamy Sabari Arul
Publisher : Springer
ISBN 13 : 9811390452
Total Pages : 355 pages
Book Rating : 4.8/5 (113 download)

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Book Synopsis Two Dimensional Transition Metal Dichalcogenides by : Narayanasamy Sabari Arul

Download or read book Two Dimensional Transition Metal Dichalcogenides written by Narayanasamy Sabari Arul and published by Springer. This book was released on 2019-07-30 with total page 355 pages. Available in PDF, EPUB and Kindle. Book excerpt: This book presents advanced synthesis techniques adopted to fabricate two-dimensional (2D) transition metal dichalcogenides (TMDs) materials with its enhanced properties towards their utilization in various applications such as, energy storage devices, photovoltaics, electrocatalysis, electronic devices, photocatalysts, sensing and biomedical applications. It provides detailed coverage on everything from the synthesis and properties to the applications and future prospects of research in 2D TMD nanomaterials.

Two-Dimensional Transition-Metal Dichalcogenides

Author : Chi Sin Tang
Publisher : John Wiley & Sons
ISBN 13 : 3527350640
Total Pages : 357 pages
Book Rating : 4.5/5 (273 download)

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Book Synopsis Two-Dimensional Transition-Metal Dichalcogenides by : Chi Sin Tang

Download or read book Two-Dimensional Transition-Metal Dichalcogenides written by Chi Sin Tang and published by John Wiley & Sons. This book was released on 2023-11-14 with total page 357 pages. Available in PDF, EPUB and Kindle. Book excerpt: Two-Dimensional Transition-Metal Dichalcogenides Comprehensive resource covering rapid scientific and technological development of polymorphic two-dimensional transition-metal dichalcogenides (2D-TMDs) over a range of disciplines and applications Two-Dimensional Transition-Metal Dichalcogenides: Phase Engineering and Applications in Electronics and Optoelectronics provides a discussion on the history of phase engineering in 2D-TMDs as well as an in-depth treatment on the structural and electronic properties of 2D-TMDs in their respective polymorphic structures. The text addresses different forms of in-situ synthesis, phase transformation, and characterization methods for 2D-TMD materials and provides a comprehensive treatment of both the theoretical and experimental studies that have been conducted on 2D-TMDs in their respective phases. Two-Dimensional Transition-Metal Dichalcogenides includes further information on: Thermoelectric, fundamental spin-orbit structures, Weyl semi-metallic, and superconductive and related ferromagnetic properties that 2D-TMD materials possess Existing and prospective applications of 2D-TMDs in the field of electronics and optoelectronics as well as clean energy, catalysis, and memristors Magnetism and spin structures of polymorphic 2D-TMDs and further considerations on the challenges confronting the utilization of TMD-based systems Recent progress of mechanical exfoliation and the application in the study of 2D materials and other modern opportunities for progress in the field Two-Dimensional Transition-Metal Dichalcogenides provides in-depth review introducing the electronic properties of two-dimensional transition-metal dichalcogenides with updates to the phase engineering transition strategies and a diverse range of arising applications, making it an essential resource for scientists, chemists, physicists, and engineers across a wide range of disciplines.

Investigation Of Electronic Structure Of Transition Metal Oxides Exhibiting Metal-insulator Transitions And Related Phenomena

Author :
Publisher :
ISBN 13 :
Total Pages : pages
Book Rating : 4.:/5 (656 download)

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Book Synopsis Investigation Of Electronic Structure Of Transition Metal Oxides Exhibiting Metal-insulator Transitions And Related Phenomena by :

Download or read book Investigation Of Electronic Structure Of Transition Metal Oxides Exhibiting Metal-insulator Transitions And Related Phenomena written by and published by . This book was released on 2002 with total page pages. Available in PDF, EPUB and Kindle. Book excerpt: Transition metal oxides have proven to be a fertile research area for condensed matter physicists due to the fascinating array of superconducting, magnetic and electronic properties they exhibit. A particular resurgence of intense activity in investigating the properties of these systems followed the discovery of high temperature superconductivity in the cuprates, colossal magnetoresistance in the manganites, ferroelectricity in the cobaltites and simultaneous ferroelectric and ferromagnetic ordering in the manganites. These diverse properties of transition metal compounds arise due to the presence of strong electron-electron interactions within the transition element 3d states. Indeed, it is the competition between the localizing effects of such interactions and the comparable hopping strengths driving the system towards delocalization, that is responsible for these wide spectrum of interesting properties. In terms of theoretical and fundamental issues, electronic structure of transition metal oxides play a most important role, providing a testing ground for new many-body theoretical approaches treating the correlation problem at various levels of approximations. In addition to this rich spectrum of properties, metal-insulator transitions often occur and can even be coincident with structural or magnetic changes due to the strong coupling between charge, magnetic and lattice degrees of freedom. However, in spite of the immense activities in this area, the underlying phenomena is not yet completely understood. A careful investigation of the electronic structure of these systems will help in the microscopic understanding of these and photoelectron spectroscopy has been established as the most powerful tool for investigating the electronic structures of these systems. In this thesis we investigate the electronic structures of some of these transition metal oxides and the metal-insulator transition as a function of electron correlation strength and doping of charge car.

Electronically highly correlated ternary transition metal oxides

Author : Alexander Krimmel
Publisher : diplom.de
ISBN 13 : 3832486925
Total Pages : 124 pages
Book Rating : 4.8/5 (324 download)

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Book Synopsis Electronically highly correlated ternary transition metal oxides by : Alexander Krimmel

Download or read book Electronically highly correlated ternary transition metal oxides written by Alexander Krimmel and published by diplom.de. This book was released on 2005-04-15 with total page 124 pages. Available in PDF, EPUB and Kindle. Book excerpt: Introduction: Transition metal oxides represent a large class of compounds with a uniquely wide range of electronic properties. Some of these properties, like the magnetism of loadstone, have been known since antiquity. Others, like high-temperature superconductivity have been discovered only recently and indeed would have been thought of being impossible 20 years ago. Transition metal oxides may be good insulators, semiconductors, metals or superconductors. Many of them display a metal-to-insulator transition (MIT) as a function of an external control parameter (usually temperature, pressure or chemical composition). The differences of electrical conductivity are also reflected by drastic changes of other physical properties related to the electronic structure. The electrical, magnetic and optical properties of transition metal oxides find a rich field of important technical applications. A classical example is the wide use of ferrites in electronic devices. Further examples of suitable technological applications include wide gap semiconductors, superconductors and thermoelectric materials, to mention just a few. Apart from these exciting electronic properties, some transition metal oxides exhibit a remarkable mechanical and high-temperature stability together with a strong resistance against corrosion, thus forming ideal coating materials. Several transition metal oxides may also serve as catalysts. It was the discovery of high-temperature superconductivity in the cuprates and, subsequently, of the colossal magneto-resistance effect (CMR) in the manganates that triggered a tremendous research effort in transition metal oxides during the last decade. [...]

Electronic Structure and Properties

Author : Frank Y. Fradin
Publisher : Elsevier
ISBN 13 : 1483218279
Total Pages : 461 pages
Book Rating : 4.4/5 (832 download)

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Book Synopsis Electronic Structure and Properties by : Frank Y. Fradin

Download or read book Electronic Structure and Properties written by Frank Y. Fradin and published by Elsevier. This book was released on 2013-10-22 with total page 461 pages. Available in PDF, EPUB and Kindle. Book excerpt: Treatise on Materials Science and Technology, Volume 21: Electronic Structure and Properties covers the developments in electron theory and electron spectroscopies. The book discusses the electronic structure of perfect and defective solids; the photoelectron spectroscopy as an electronic structure probe; and the electron-phonon interaction. The text describes the elastic properties of transition metals; the electrical resistivity of metals; as well as the electronic structure of point defects in metals. Metallurgists, materials scientists, materials engineers, and students involved in the related fields will find the book useful.

Two-Dimensional Transition-Metal Dichalcogenides

Author : Alexander V. Kolobov
Publisher : Springer
ISBN 13 : 3319314505
Total Pages : 545 pages
Book Rating : 4.3/5 (193 download)

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Book Synopsis Two-Dimensional Transition-Metal Dichalcogenides by : Alexander V. Kolobov

Download or read book Two-Dimensional Transition-Metal Dichalcogenides written by Alexander V. Kolobov and published by Springer. This book was released on 2016-07-26 with total page 545 pages. Available in PDF, EPUB and Kindle. Book excerpt: This book summarizes the current status of theoretical and experimental progress in 2 dimensional graphene-like monolayers and few-layers of transition metal dichalcogenides (TMDCs). Semiconducting monolayer TMDCs, due to the presence of a direct gap, significantly extend the potential of low-dimensional nanomaterials for applications in nanoelectronics and nano-optoelectronics as well as flexible nano-electronics with unprecedented possibilities to control the gap by external stimuli. Strong quantum confinement results in extremely high exciton binding energies which forms an interesting platform for both fundamental studies and device applications. Breaking of spatial inversion symmetry in monolayers results in strong spin-valley coupling potentially leading to their use in valleytronics. Starting with the basic chemistry of transition metals, the reader is introduced to the rich field of transition metal dichalcogenides. After a chapter on three dimensional crystals and a description of top-down and bottom-up fabrication methods of few-layer and single layer structures, the fascinating world of two-dimensional TMDCs structures is presented with their unique atomic, electronic, and magnetic properties. The book covers in detail particular features associated with decreased dimensionality such as stability and phase-transitions in monolayers, the appearance of a direct gap, large binding energy of 2D excitons and trions and their dynamics, Raman scattering associated with decreased dimensionality, extraordinarily strong light-matter interaction, layer-dependent photoluminescence properties, new physics associated with the destruction of the spatial inversion symmetry of the bulk phase, spin-orbit and spin-valley couplings. The book concludes with chapters on engineered heterostructures and device applications such as a monolayer MoS2 transistor. Considering the explosive interest in physics and applications of two-dimensional materials, this book is a valuable source of information for material scientists and engineers working in the field as well as for the graduate students majoring in materials science.

Electronic Structure and Properties of Transition Metal Compounds

Author : Isaac B. Bersuker
Publisher : Wiley-Interscience
ISBN 13 :
Total Pages : 698 pages
Book Rating : 4.:/5 (319 download)

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Book Synopsis Electronic Structure and Properties of Transition Metal Compounds by : Isaac B. Bersuker

Download or read book Electronic Structure and Properties of Transition Metal Compounds written by Isaac B. Bersuker and published by Wiley-Interscience. This book was released on 1996-03-28 with total page 698 pages. Available in PDF, EPUB and Kindle. Book excerpt: Covering all the latest developments, and applying the theory of electronic structure to problem solving at every opportunity, Electronic Structure and Properties of Transition Metal Compounds places the reader at the cutting edge of this important field of research. The book focuses on the electronic structure and related properties of coordination compounds, essentially treating chemical bonding as an electronic phenomenon. It also covers the central concepts of quantum chemistry and atomic states, examines theories of electronic structure and vibronic coupling, and explores physical methods of investigation. The applications of the theory to stereochemistry and crystal chemistry, electron transfer and electron-conformational effects, and reactivity and catalytic action are also discussed.

A Comparative Study of 3d-intercalated Transition Metal Dichalcogenides by Magnetic, Transport, and Electronic Properties

Author : Deepak Sapkota (Researcher in physics)
Publisher :
ISBN 13 :
Total Pages : 0 pages
Book Rating : 4.:/5 (141 download)

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Book Synopsis A Comparative Study of 3d-intercalated Transition Metal Dichalcogenides by Magnetic, Transport, and Electronic Properties by : Deepak Sapkota (Researcher in physics)

Download or read book A Comparative Study of 3d-intercalated Transition Metal Dichalcogenides by Magnetic, Transport, and Electronic Properties written by Deepak Sapkota (Researcher in physics) and published by . This book was released on 2019 with total page 0 pages. Available in PDF, EPUB and Kindle. Book excerpt: Intercalation of transition metal dichalcogendies (TMDCs) by 3d-transition metals has been studied systematically. We mainly focus on intercalation into two host TMDCs 2H-NbS2 and 2H-TaS2 which are layered materials where the metal ions are in trigonal prismatic environment of chalcogens, the layers are separated by weak van der Waals force. So, foreign atoms or molecules can be inserted in between the layers of the TMDCs. The un-intercalated NbS2 shows superconductivity below 6 K whereas TaS2 exhibits coexistence of the superconductivity (Tc̳=0.8 K) with charge density wave phase (TC̳D̳W̳=75 K). In this research, the NbS2 is intercalated by V atom with formula unit V0.3NbS2, while TaS2 by Cr with formula unit Cr1/3TaS2. Upon the intercalation, the electronic as well as magnetic structure of host materials are likely to be modified. It is believed that the charge transfer between the 3d-intercalant and host TMDC, specifically the d-band of Nb or Ta, just causes an increase in chemical potential without altering the band structure and shape and size of Fermi surface, also known as rigid band model. And, the local moment in magnetic ion gives rise to magnetism via RKKY interaction. In order to examine the effect of intercalation in V0.3NbS2 and Cr1/3TaS2, we investigated the magnetic, transport, and electronic properties. In V0.3NbS2, which crystallizes in P-31m space group, we observed canted antiferromag-netic (weak ferromagnetic) magnetic ordering with majority of charge carriers as hole type. From ARPES measurements, additional bands are appeared to cross the Fermi level and shape and size of the Fermi surface are modified as compared to NbS2. Also, V-3d states are present near the Fermi level. These findings demonstrate that the simple rigid band picture is not viable in V0.3NbS2 compound. Moreover, from the photon dependent ARPES measurements strong kz̳ dispersion is found in contrast to that of host NbS2. Similarly, intercalated Cr1/3TaS2 crystallizes in P6322 space group orders ferromagnetically. Surface structure is investigated by STM, LEED, and core level photoemmission experiments. The resonant photoemmission and ARPES measurements are performed to examine the effect of charge transfer between Cr and TaS2 layer.

Energy Research Abstracts

Author :
Publisher :
ISBN 13 :
Total Pages : 1684 pages
Book Rating : 4.U/5 (183 download)

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Book Synopsis Energy Research Abstracts by :

Download or read book Energy Research Abstracts written by and published by . This book was released on 1988 with total page 1684 pages. Available in PDF, EPUB and Kindle. Book excerpt:

Nuclear Science Abstracts

Author :
Publisher :
ISBN 13 :
Total Pages : 964 pages
Book Rating : 4.3/5 (91 download)

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Book Synopsis Nuclear Science Abstracts by :

Download or read book Nuclear Science Abstracts written by and published by . This book was released on 1976 with total page 964 pages. Available in PDF, EPUB and Kindle. Book excerpt:

2D Materials

Author : Phaedon Avouris
Publisher : Cambridge University Press
ISBN 13 : 1107163714
Total Pages : 521 pages
Book Rating : 4.1/5 (71 download)

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Book Synopsis 2D Materials by : Phaedon Avouris

Download or read book 2D Materials written by Phaedon Avouris and published by Cambridge University Press. This book was released on 2017-06-29 with total page 521 pages. Available in PDF, EPUB and Kindle. Book excerpt: A comprehensive and accessible introduction to 2D materials, covering basic physics, electronic and optical properties, and potential applications.

Transition Metal Oxides

Author : P. A. Cox
Publisher : Oxford University Press
ISBN 13 : 0191030139
Total Pages : 295 pages
Book Rating : 4.1/5 (91 download)

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Book Synopsis Transition Metal Oxides by : P. A. Cox

Download or read book Transition Metal Oxides written by P. A. Cox and published by Oxford University Press. This book was released on 2010-08-19 with total page 295 pages. Available in PDF, EPUB and Kindle. Book excerpt: Transition metal oxides form a series of compounds with a uniquely wide range of electronic properties. They have important applications as dielectrics,semiconductors, and metals, and as materials for magnetic and optical uses. The recent discovery of `high temperature' superconductors has brought the attention of a wide scientific community to this area and has highlighted the problems involved in trying to understand transition metal oxides. The present book is not primarily about Tc superconductors, although their main properties are discussed in the final sections. The main aim is to describe the varied electronic behaviour shown by transition metal oxides, and to discuss the different types of theoretical model that have been proposed to interpret it. It is intended to provide an introduction to this fascinating and difficult field, at a level suitable for graduate students and other research workers with a background in solid- state chemistry or physics.

Electron Density

Author : Pratim Kumar Chattaraj
Publisher : John Wiley & Sons
ISBN 13 : 1394217625
Total Pages : 613 pages
Book Rating : 4.3/5 (942 download)

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Book Synopsis Electron Density by : Pratim Kumar Chattaraj

Download or read book Electron Density written by Pratim Kumar Chattaraj and published by John Wiley & Sons. This book was released on 2024-09-30 with total page 613 pages. Available in PDF, EPUB and Kindle. Book excerpt: Discover theoretical, methodological, and applied perspectives on electron density studies and density functional theory Electron density or the single particle density is a 3D function even for a many-electron system. Electron density contains all information regarding the ground state and also about some excited states of an atom or a molecule. All the properties can be written as functionals of electron density, and the energy attains its minimum value for the true density. It has been used as the basis for a quantum chemical computational method called Density Functional Theory, or DFT, which can be used to determine various properties of molecules. DFT brings out a drastic reduction in computational cost due to its reduced dimensionality. Thus, DFT is considered to be the workhorse for modern computational chemistry, physics as well as materials science. Electron Density: Concepts, Computation and DFT Applications offers an introduction to the foundations and applications of electron density studies and analysis. Beginning with an overview of major methodological and conceptual issues in electron density, it analyzes DFT and its major successful applications. The result is a state-of-the-art reference for a vital tool in a range of experimental sciences. Readers will also find: A balance of fundamentals and applications to facilitate use by both theoretical and computational scientists Detailed discussion of topics including the Levy-Perdew-Sahni equation, the Kohn Sham Inversion problem, and more Analysis of DFT applications including the determination of structural, magnetic, and electronic properties Electron Density: Concepts, Computation and DFT Applications is ideal for academic researchers in quantum, theoretical, and computational chemistry and physics.

Spin-orbit Coupling Effects in Two-Dimensional Electron and Hole Systems

Author : Roland Winkler
Publisher : Springer Science & Business Media
ISBN 13 : 9783540011873
Total Pages : 244 pages
Book Rating : 4.0/5 (118 download)

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Book Synopsis Spin-orbit Coupling Effects in Two-Dimensional Electron and Hole Systems by : Roland Winkler

Download or read book Spin-orbit Coupling Effects in Two-Dimensional Electron and Hole Systems written by Roland Winkler and published by Springer Science & Business Media. This book was released on 2003-10-10 with total page 244 pages. Available in PDF, EPUB and Kindle. Book excerpt: The first part provides a general introduction to the electronic structure of quasi-two-dimensional systems with a particular focus on group-theoretical methods. The main part of the monograph is devoted to spin-orbit coupling phenomena at zero and nonzero magnetic fields. Throughout the book, the main focus is on a thorough discussion of the physical ideas and a detailed interpretation of the results. Accurate numerical calculations are complemented by simple and transparent analytical models that capture the important physics.

Electronic Properties of Surfaces

Author : Prutton
Publisher : Routledge
ISBN 13 : 1351453041
Total Pages : 232 pages
Book Rating : 4.3/5 (514 download)

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Book Synopsis Electronic Properties of Surfaces by : Prutton

Download or read book Electronic Properties of Surfaces written by Prutton and published by Routledge. This book was released on 2018-02-06 with total page 232 pages. Available in PDF, EPUB and Kindle. Book excerpt: In recent years the availability of techniques and the asking of basic and technological questions has led to an international explosion of activity in the study of solid surfaces. Originally published in Reports in Progress in Physics, Electronic Properties of Surfaces reflects the modern knowledge in this field, presenting critical appraisals of progress in surface science. The book should be particularly valuable for researchers new to this field.