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Design And Development Of A New Generation Of Uv Visible Light Driven Nanosized Codoped Titanium Dioxide Photocatalysts And Biocides Sporocides And Environmental Applications
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Book Synopsis Design and Development of a New Generation of UV-visible-light-driven Nanosized Codoped Titanium Dioxide Photocatalysts and Biocides/sporocides, and Environmental Applications by :
Download or read book Design and Development of a New Generation of UV-visible-light-driven Nanosized Codoped Titanium Dioxide Photocatalysts and Biocides/sporocides, and Environmental Applications written by and published by . This book was released on 2009 with total page pages. Available in PDF, EPUB and Kindle. Book excerpt: For solar environmental remediation, a new generation of nanosized (10 nm) titanium dioxide photocatalysts codoped with metals and nonmetals, or metals only were prepared by the xero-gel and aero-gel methods. For silver or cobalt-based xero-gel titanium dioxide photocatalysts, photoactivities tests revealed that codoping of titanium dioxide with a metal (1% Ag or 2% Co) and nonmetals (carbon and sulfur) is necessary to achieve high-activities for acetaldehyde degradation under visible light (wavelength 420 nm). It was concluded that high visible-light-activities for acetaldehyde degradation over codoped titanium dioxide were attributed to an interplay of anatase crystallinity, high-surface area, reduced band-gap (3.0 eV), uniform dispersion of doped metal ions, and suppressed recombination rate of photogenerated electron-hole pairs. Moreover, the nature and amount of codoped metals play a significant role in visible-light-induced photocatalysis. Metals (Al, Ga, and In) doped/codoped titanium dioxide photocatalysts were prepared by the aero-gel method. The photocatalytic studies showed that activities of metal doped/codoped photocatalysts under UV light (wavelength 400 nm) were found to be dependent on pollutants. Indium demonstrated beneficial effects in both textural and photocatalytic properties. Gallium and indium codoped titanium dioxide photocatalysts displayed even better performance in the CO oxidation reaction under UV light. Notably, titanium dioxide codoped with Ga, In, and Pt, exhibited unique photoactivities for the CO oxidation under both UV and visible light irradiation, indicating that this system could have promise for the water-gas shift reaction for hydrogen production. Silver-based nanostructured titanium dioxide samples were developed for killing human pathogens (Escherichia coli cells and Bacillus subtilis spores). Biocidal tests revealed that silver, carbon, and sulfur codoped titanium dioxide nanoparticles (
Book Synopsis Visible-Light-Active Photocatalysis by : Srabanti Ghosh
Download or read book Visible-Light-Active Photocatalysis written by Srabanti Ghosh and published by John Wiley & Sons. This book was released on 2018-03-23 with total page 626 pages. Available in PDF, EPUB and Kindle. Book excerpt: A comprehensive and timely overview of this important and hot topic, with special emphasis placed on environmental applications and the potential for solar light harvesting. Following introductory chapters on environmental photocatalysis, water splitting, and applications in synthetic chemistry, further chapters focus on the synthesis and design of photocatalysts, solar energy conversion, and such environmental aspects as the removal of water pollutants, photocatalytic conversion of CO2. Besides metal oxide-based photocatalysts, the authors cover other relevant material classes including carbon-based nanomaterials and novel hybrid materials. Chapters on mechanistic aspects, computational modeling of photocatalysis and Challenges and perspectives of solar reactor design for industrial applications complete this unique survey of the subject. With its in-depth discussions ranging from a comprehensive understanding to the engineering of materials and applied devices, this is an invaluable resource for a range of disciplines.
Book Synopsis Environmentally Benign Photocatalysts by : Masakazu Anpo
Download or read book Environmentally Benign Photocatalysts written by Masakazu Anpo and published by Springer Science & Business Media. This book was released on 2010-11-10 with total page 740 pages. Available in PDF, EPUB and Kindle. Book excerpt: Over the past few decades, mankind has observed an unprecedented and remarkable growth in industry, resulting in a more prosperous lifestyle for peoples of many countries. In developing countries, however, explosive industrial growth is just now beginning to raise the living standards of the people. Most industries, especially in these developing countries, are still powered by the burning of fossil fuels; con- quently, a lack of clean energy resources has caused environmental pollution on an unprecedented large and global scale. Toxic wastes have been relentlessly released into the air and water leading to serious and devastating environmental and health problems while endangering the planet and life itself with the effects of global warming. To address these urgent environmental issues, new catalytic and photocatalytic processes as well as open-atmospheric systems are presently being developed that can operate at room temperature while being totally clean and ef?cient and thus environmentally harmonious. Essential to technologies harnessing the abundant solar energy that reaches the earth are the highly functional photocatalytic proce- es that can utilize not only UV light, but also visible light.
Book Synopsis Nanosized Titania Composites for Reinforcement of Photocatalysis and Photoelectrocatalysis by : Maksym Zahornyi
Download or read book Nanosized Titania Composites for Reinforcement of Photocatalysis and Photoelectrocatalysis written by Maksym Zahornyi and published by Cambridge Scholars Publishing. This book was released on 2022-02-06 with total page 275 pages. Available in PDF, EPUB and Kindle. Book excerpt: This book discusses recent advances in the photocatalytic and electrophotocatalytic applications of titanium dioxide nanocomposites containing polymers and other components. These materials possess photocatalytic, virucidal and antimicrobial efficacy and water and air cleaning abilities against eco-toxicants, and allow water splitting for the generation of chemical fuels. The book considers the ability of nanocomposites’ components to reinforce titania functionality in photocatalysis and photoelectrocatalysis, and presents an overview of their occurrence in nature, their thermodynamic properties, and their toxicity. The volume will be of interest to chemists and material science specialists and practitioners, as well as any reader interested in the recent scientific achievements for green and sustainable development.
Book Synopsis Nanostructured Titanium Dioxide in Photocatalysis by : It-Meng Low
Download or read book Nanostructured Titanium Dioxide in Photocatalysis written by It-Meng Low and published by CRC Press. This book was released on 2021-06-18 with total page 320 pages. Available in PDF, EPUB and Kindle. Book excerpt: Titanium dioxide (TiO2) has drawn considerable attention as an attractive inorganic raw material for various applications due to its inexpensiveness, nontoxic nature, stability, and excellent photocatalytic activity. Photocatalysis is one of the most promising route for sustainable chemistry of the 21st century. It can contribute to solving environmental, global energy, and chemical problems, as well as to the sustainable production of commodities in the near future. This book presents the fundamentals of photocatalysis in nanostructured TiO2 and describes the factors affecting the photocatalytic activity, design, and synthesis of various forms of nanostructured TiO2. It highlights the use of ion-doping and inert-atmosphere annealing to extend the light-absorption range of photocatalysts and reduce recombination between electrons and holes. It discusses numerous applications in the fields of energy and environment, such as water purification, gas sensing, storage and delivery, and energy generation. The book is an invaluable resource and useful guide for a broad readership in various fields of catalysis, materials science, environment, and energy.
Book Synopsis Photocatalytic Activity Enhancement of Titanium Dioxide Nanoparticles by : Mohamed A. Barakat
Download or read book Photocatalytic Activity Enhancement of Titanium Dioxide Nanoparticles written by Mohamed A. Barakat and published by Springer. This book was released on 2015-10-26 with total page 39 pages. Available in PDF, EPUB and Kindle. Book excerpt: In this brief, a comprehensive review of the UV/visible-TiO2 photocatalytic oxidation process is presented with an insight into the mechanisms involved, the role of titanium dioxide as a catalyst, irradiation sources, types of reactors, and a comparison between various modes of TiO2 application. An overview of the development and enhancement of the activity of TiO2 nanoparticles in photocatalysis is presented. The topics covered include a detailed look at the unique properties of the TiO2 nanoparticles and their relationship to photocatalytic properties. The utilization of the TiO2 nanoparticles as photocatalysts, in the non-doped and doped forms is also reviewed. Finally, the use of modified TiO2 nanoparticles has made a significant contribution in providing definitive mechanistic information regarding the visible light photocatalytic processes.
Download or read book Titanium Dioxide written by Dongfang Yang and published by BoD – Books on Demand. This book was released on 2018-06-27 with total page 520 pages. Available in PDF, EPUB and Kindle. Book excerpt: Titanium dioxide is currently being used in many industrial products. It provides unique photocatalytic properties for water splitting and purification, bacterial inactivation, and organics degradation. It has also been widely used as the photoanode for dye-sensitized solar cells and coatings for self-cleaning surfaces, biomedical implants, and nanomedicine. This book covers various aspects of titanium dioxide nanomaterials including their unique one-dimensional, two-dimensional, mesoporous, and hierarchical nanostructures and their synthetic methods such as sol-gel, hydrothermal, anodic oxidation, and electrophoretic deposition, as well as its key applications in environmental and energy sectors. Through these 24 chapters written by experts from the international scientific community, readers will have access to a comprehensive overview of the recent research and development findings on the titanium dioxide nanomaterials.
Book Synopsis Titanium Dioxide Photocatalysis by : Vladimiro Dal Santo
Download or read book Titanium Dioxide Photocatalysis written by Vladimiro Dal Santo and published by MDPI. This book was released on 2019-05-27 with total page 208 pages. Available in PDF, EPUB and Kindle. Book excerpt: Although the seminal work of Fujishima et al. dates back to 1971, TiO2 still remains the most diffused and studied semiconductor, employed in photo-oxidation processes for cleantech (i.e., polluted water and air treatment), in solar fuel production (mainly hydrogen production by water photo splitting), and in Carbon Capture and Utilization (CCU) processes by CO2 photoreduction. The eleven articles, among them three reviews, in this book cover recent results and research trends of various aspects of titanium dioxide photocatalysis, with the chief aim of improving the final efficiency of TiO2-based materials. Strategies include doping, metal co-catalyst deposition, and the realization of composites with plasmonic materials, other semiconductors, and graphene. Photocatalysts with high efficiency and selectivity can be also obtained by controlling the precise crystal shape (and homogeneous size) and the organization in superstructures from ultrathin films to hierarchical nanostructures. Finally, the theoretical modeling of TiO2 nanoparticles is discussed and highlighted. The range of topics addressed in this book will stimulate the reader’s interest as well as provide a valuable source of information for researchers in academia and industry.
Book Synopsis Environmentally Benign Photocatalysts by : Masakazu Anpo
Download or read book Environmentally Benign Photocatalysts written by Masakazu Anpo and published by Springer. This book was released on 2016-04-01 with total page 772 pages. Available in PDF, EPUB and Kindle. Book excerpt: Titanium oxide-based catalysts show promise as a stable, non-toxic photofunctional material. This book covers approaches in the design of titanium oxide-based photocatalysts: sol-gel, precipitation, dip-coating, metal implantation and sputtering deposition.
Book Synopsis Development of Novel Visible and Solar Light-activated Nanostructured Nitrogen-fluorine Titanium Dioxide Photocatalyst for the Removal of Cyanotoxins in Water by : Miguel Pelaez
Download or read book Development of Novel Visible and Solar Light-activated Nanostructured Nitrogen-fluorine Titanium Dioxide Photocatalyst for the Removal of Cyanotoxins in Water written by Miguel Pelaez and published by . This book was released on 2012 with total page 203 pages. Available in PDF, EPUB and Kindle. Book excerpt: The prevalent and increasing occurrence of cyanobacteria and their toxins, known as cyanotoxins, in drinking water sources have become a potential health risk to humans. Physical treatment methods in conventional drinking water treatment have the capacity to remove cyanotoxins but are limited to a merely physical separation, where further treatment is required. Cyanotoxins are susceptible to chemical oxidation and recently advanced oxidation technologies (AOTs) and nanotechnologies (AONs), such as titanium dioxide (TiO2) photocatalysis, have been proven an effective alternative technology to chemically transform cyanotoxins in water. However, conventional TiO2 is restricted to UV light photoactivation for the generation of highly reactive oxygen species (i.e., hydroxyl radicals) representing an economical and technological limitation for the use of renewable energy sources such as solar light, since UV radiation accounts only for 5% of the total solar spectrum compared to the visible spectrum (~45%). This dissertation explored the development of nanostructured nitrogen and fluorine co-doped TiO2 (NF-TiO2) that can be activated under visible and solar light for the photocatalytic degradation of cyanotoxins in water. This work aimed to develop highly efficient NF-TiO2 nanoparticles and films to evaluate the environmental fate of microcystins, the most widespread and highly persistent group of cyanotoxins found in surface waters, and cylindrospermopsin which has emerged as the most significant toxin in freshwater sources. Specific attention was given to 1) the fundamental aspects on the synthesis method that influenced the physicochemical properties of NF-TiO2, such as the incorporation of nitrogen and fluorine in the structure of TiO2 and the synergistic effects induced by both dopants, 2) the surface interaction between the cyanotoxins and NF-TiO2 in different water matrix, 3) the reactivity and degradation kinetics of microcystins and cylindrospermopsin with NF-TiO2 and 4) the mechanism of radical formation with NF-TiO2 under visible and solar light. The existence of interstitial nitrogen and substitutional fluorine in the NF-TiO2 lattice was determined and the formation of localized intra-gap states was established implying that fluorine promotes nitrogen incorporation in TiO2. A shift in the absorbance capacity of NF-TiO2 in the visible range was also observed. Anatase/brookite heterojunctions, which promote photocatalytic efficiency, were found in NF-TiO2. High initial degradation rates for microcystin-LR (MC-LR) were obtained with NF-TiO2 nanoparticles and films in synthetic water under visible light. The effect of pH indicated that attractive forces at acidic conditions between the oppositely charged NF-TiO2 and MC-LR contributed to higher MC-LR initial degradation rates. The presence of alkalinity and natural organic matter had a scavenging effect since the initial MC-LR degradation rates decreased. Modifications to NF-TiO2 with Evonik Aeroxide P25-TiO2 (P25) nanoparticles lead to composite NF-TiO2-P25 with improved photocatalytic activity towards MC-LR, MC-RR, MC-YR, MC-LA and cylindrospermopsin under visible and UV-vis light. The general reactivity was MC-LA>MC-LR>MC-YR>MC-RR. Finally, results using selected scavengers indicate that the main mechanism of NF-TiO2 radical formation under visible light irradiation differed from UV-mediated TiO2 photocatalysis since no evidence of hydroxyl radical production from the surface holes was observed. It was suggested that under visible light, surface oxygen reduction of NF-TiO2 occurred to form superoxide radical anion as main radical specie. The affinity of the scavenger with NF-TiO2 and MC-LR in terms of pH was established as an important parameter to determine the radicals formed in this study.
Book Synopsis Titanium Dioxide by : Aparna B. Gunjal
Download or read book Titanium Dioxide written by Aparna B. Gunjal and published by Nova Science Publishers. This book was released on 2021 with total page 138 pages. Available in PDF, EPUB and Kindle. Book excerpt: This book, titled Titanium Dioxide: Advances in Research and Applications, deals with important aspects of applications of titanium dioxide and recent developments in the areas of research of titanium dioxide. There are 5 chapters in this book contributed by various authors. Chapter 1 deals with applications of titanium dioxide in space and its photocatalytic activity in a vacuum environment. Chapter 2 mentions various applications of titanium dioxide in the biomedical field, such as in bone implantation, immobilization of drug carriers, and in cancer therapy as well as in environmental remediation, such as degradation of hazardous pollutants and treatment of wastewater. Chapter 3 deals with doped titanium dioxide nanostructures for visible light driven photo catalysis. The applications of visible light on active titanium dioxide photocatalysts for degradation of various toxic pollutants are described. Chapter 4 deals in detail with various methods of biosynthesis of titanium dioxide nanoparticles and their antibacterial activity. Chapter 5 describes preparation of titanium dioxide nonmaterials, their forensic applications, and fingerprint imaging. The book Titanium Dioxide: Advances in Research and Applications will be of immense use to students, professors and researchers of various colleges, universities and research institutes. It will increase knowledge regarding the synthesis, applications and various aspects of titanium dioxide.
Book Synopsis Nanostructured Photocatalysts by : Hiromi Yamashita
Download or read book Nanostructured Photocatalysts written by Hiromi Yamashita and published by Springer. This book was released on 2016-05-03 with total page 543 pages. Available in PDF, EPUB and Kindle. Book excerpt: While books on semiconductor TiO2 photocatalysis are legion, nanostructured controlled photocatalysts are attractive beyond standard semiconductors, and this book is devoted to the many novel uses of advanced TiO2 and MOF-based photocatalysts. Details on synthesis, characterization, and reaction applications of nanostructured photocatalysts are summarized. Other new materials discussed in this book are Bi- W- oxides, metal complexes, and unique porous materials. This book contains methods of preparation and characterization of unique nanostructured photocatalysts, and details about their catalytic action. Contributors to this volume are leading Asian researchers in Photocatalysis. It will appeal to researchers wishing to know how to design new types of photocatalysts with controlled nanostructures.
Book Synopsis Novel Preparation of Nanostructured Titanium Dioxide Photocatalytic Particles, Films, Membranes, and Devices for Environmental Applications by : Hyeok Choi
Download or read book Novel Preparation of Nanostructured Titanium Dioxide Photocatalytic Particles, Films, Membranes, and Devices for Environmental Applications written by Hyeok Choi and published by . This book was released on 2007 with total page 249 pages. Available in PDF, EPUB and Kindle. Book excerpt: From a scientific point of view, this study will provide new nanotechnological and materials chemistry procedures to synthesize highly efficient photocatalytic TiO2 particles, films, and membranes that can be used for the treatment and disinfection of water and wastewater under even visible light irradiation, and highly sensitive TiO2-based devices for the development of new type of sensors.
Book Synopsis Improving the Optoelectronic Property and Photoactivity of Nano-structured Titanuim Dioxide by : Hong-Ying Lin
Download or read book Improving the Optoelectronic Property and Photoactivity of Nano-structured Titanuim Dioxide written by Hong-Ying Lin and published by ProQuest. This book was released on 2008 with total page pages. Available in PDF, EPUB and Kindle. Book excerpt: Titanium dioxide (TiO 2) has been proven to be one of the most important and widely used photocatalyst for applications such as gas/liquid phase environmental cleaning, solar hydrogen generation, sensitized solar cell, UV filtration, etc. The biggest challenge in the applications of this semiconductor photocatalyst is its large band gap (~ 3.2 eV) which limits the utilizable spectrum of photons from the solar light (~ 4 to 5 %). To improve the optical sensitivity of TiO 2 in the visible light region, the band gap of TiO 2 needs to be tailored. The reduction of TiO 2 band gap can be achieved by controlling of its electronic structure via two routes: changing the particle size and doping it with impurities. To precisely control the size of TiO 2 particles, anatase TiO 2 nanocrystallines (17 to 29 nm) were synthesized by metallo-organic chemical vapor deposition (MOCVD) method with moderate control on system parameters (i.e. pressure and gas flow rates). The results of band gap change as a function of particle size agreed well with what was predicted using the Brus' effective mass model (EMM). However, the observations from photocatalytic oxidation of 2-chlorophenol (2-CP) showed that the smaller the particle size, the faster the degradation rate. This is attributed in part to the combined effect of band gap change relative to the spectrum of the light source and the specific surface area (or particle size) of the photocatalysts. Our results indicate that the gain in specific surface area due to the smaller particle size outweighs the improvement on its optical property (e.g. reduction in bandgap) under similar experimental condition. Our observation also showed the secondary particle size to be time dependent due to the aggregation and is highly correlated with its primary particle size. The nitrogen doped TiO 2 thin film synthesis was carried out with two different approaches: (1) oxidation of the titanium nitride (TiN) thin film and (2) reactive pulsed laser deposition (PLD). Nitrogen doping of TiO 2 in the former approach was done by the oxidation of TiN thin films at 800 ̊C in ambient air. The phase transformation of TiN to TiO 2 appears to be a function of annealing time. The X-ray photoelectron spectroscopy (XPS) studies have shown that the substitutionally doped TiO 2-x N x (N 1 s ~ 396 eV) remains stable only for the first two minutes of annealing. As the annealing proceeds, the N 1s XPS peak shifts to higher binding energy (N1 s ~ 400 and 402 eV) which indicates that binding energy of N atom shifted from substitutional site (Ti-N) to chemisorbed site (N=-N) when annealing process exceeds five minutes due to the substitution of Ti-N bond by Ti-O bond. Results from both depth profile XPS and cross-section TEM showed that the formation of TiO 2-x N x depends on the distance from the film surface. Film structure studied by X-ray diffraction (XRD) showed that mixed TiN and rutile TiO 2 phases formed between four and twenty four hours of annealing time. The optical properties were examined using UV-VIS spectroscopy. The most visible light sensitive samples showed ~65 to 105 nm red-shift on its absorption edges from that of pure TiO 2, which is equivalent to ~0.47 to 0.73 eV reduction in the effective bandgap. Our results suggest that surface oxidation of TiN is an effective method for the synthesis of band gap tailored oxides which have applications in photocatalysis, photovoltaic, etc. Doping of N into TiO 2 lattice was also achieved using the reactive pulsed laser deposition technique. The N concentration was controlled by adjusting the mixing ratio of make-up (N 2) and buffer (1:1 O 2 and Ar mixture) gases during laser ablation. (Abstract shortened by UMI.).
Book Synopsis Nanostructured Titanium Dioxide Materials by : Ali Reza Khataee
Download or read book Nanostructured Titanium Dioxide Materials written by Ali Reza Khataee and published by World Scientific. This book was released on 2012 with total page 205 pages. Available in PDF, EPUB and Kindle. Book excerpt: During the past decade, research and development in the area of synthesis and applications of different nanostructured titanium dioxide have become tremendous. This book briefly describes properties, production, modification and applications of nanostructured titanium dioxide focusing in particular on photocatalytic activity. The physicochemical properties of nanostructured titanium dioxide are highlighted and the links between properties and applications are emphasized. The preparation of TiO2 nanomaterials, including nanoparticles, nanorods, nanowires, nanosheets, nanofibers, and nanotubes are primarily categorized by their preparation method (sol-gel and hydrothermal processes). Examples of early applications of nanostructured titanium dioxide in dye-sensitized solar cells, hydrogen production and storage, sensors, rechargeable batteries, electrocatalysis, self-cleaning and antibacterial surfaces and photocatalytic cancer treatment are reviewed. The review of modifications of TiO2 nanomaterials is mainly focused on the research related to the modifications of the optical properties of TiO2 nanomaterials, since many applications of TiO2 nanomaterials are closely related to their optical properties. Photocatalytic removal of various pollutants using pure TiO2 nanomaterials, TiO2-based nanoclays and non-metal doped nanostructured TiO2 are also discussed.
Book Synopsis Photocatalytic Nanomaterials for Environmental Applications by : Rajesh J. Tayade
Download or read book Photocatalytic Nanomaterials for Environmental Applications written by Rajesh J. Tayade and published by Materials Research Forum LLC. This book was released on 2018-02-25 with total page 486 pages. Available in PDF, EPUB and Kindle. Book excerpt: Photocatalytic nanomaterials have a great potential in such applications as reduction of carbon dioxide and degradation of various pollutants. They are equally important in the production and storage of energy, e.g. in the conversion of solar energy to electricity, and the production of hydrogen in photoelectrochemical cells. Research on synthesis, characterization and specific applications is reported for titanium oxide and a number of other promising catalysts, such as silver phosphate, cerium oxide, zinc oxide and zinc sulfide.
Book Synopsis Nanostructured Titanium Dioxide in Photocatalysis by : It-Meng Low
Download or read book Nanostructured Titanium Dioxide in Photocatalysis written by It-Meng Low and published by Jenny Stanford Publishing. This book was released on 2021-06-18 with total page 350 pages. Available in PDF, EPUB and Kindle. Book excerpt: Titanium dioxide (TiO2) has drawn considerable attention as an attractive inorganic raw material for various applications due to its inexpensiveness, nontoxic nature, stability, and excellent photocatalytic activity. Photocatalysis is one of the most promising route for sustainable chemistry of the 21st century. It can contribute to solving environmental, global energy, and chemical problems, as well as to the sustainable production of commodities in the near future. This book presents the fundamentals of photocatalysis in nanostructured TiO2 and describes the factors affecting the photocatalytic activity, design, and synthesis of various forms of nanostructured TiO2. It highlights the use of ion-doping and inert-atmosphere annealing to extend the light-absorption range of photocatalysts and reduce recombination between electrons and holes. It discusses numerous applications in the fields of energy and environment, such as water purification, gas sensing, storage and delivery, and energy generation. The book is an invaluable resource and useful guide for a broad readership in various fields of catalysis, materials science, environment, and energy.
