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Ultrafast Dynamics At The Nanoscale
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Book Synopsis Ultrafast Dynamics at the Nanoscale by : Stefan Haacke
Download or read book Ultrafast Dynamics at the Nanoscale written by Stefan Haacke and published by CRC Press. This book was released on 2017-01-06 with total page 529 pages. Available in PDF, EPUB and Kindle. Book excerpt: Ultrafast Dynamics at the Nanoscale provides a combined experimental and theoretical insight into the molecular-level investigation of light-induced quantum processes in biological systems and nanostructured (bio)assemblies. Topics include DNA photostability and repair, photoactive proteins, biological and artificial light-harvesting systems, plasmonic nanostructures, and organic photovoltaic materials, whose common denominator is the key importance of ultrafast quantum effects at the border between the molecular scale and the nanoscale. The functionality and control of these systems have been under intense investigation in recent years in view of developing a detailed understanding of ultrafast nanoscale energy and charge transfer, as well as fostering novel technologies based on sustainable energy resources. Both experiment and theory have made big strides toward meeting the challenge of these truly complex systems. This book, thus, introduces the reader to cutting-edge developments in ultrafast nonlinear optical spectroscopies and the quantum dynamical simulation of the observed dynamics, including direct simulations of two-dimensional optical experiments. Taken together, these techniques attempt to elucidate whether the quantum coherent nature of ultrafast events enhances the efficiency of the relevant processes and where the quantum–classical boundary sets in, in these high-dimensional biological and material systems. The chapters contain well-illustrated accounts of the authors’ research work, including didactic introductory material, and address a multidisciplinary audience from chemistry, physics, biology, and materials sciences. The book is, therefore, a must-have for graduate- and postgraduate-level researchers who wish to learn about molecular nanoscience from a combined spectroscopic and theoretical viewpoint.
Book Synopsis Ultrafast Dynamics at the Nanoscale by : Stefan Haacke
Download or read book Ultrafast Dynamics at the Nanoscale written by Stefan Haacke and published by CRC Press. This book was released on 2017-01-06 with total page 550 pages. Available in PDF, EPUB and Kindle. Book excerpt: Ultrafast Dynamics at the Nanoscale provides a combined experimental and theoretical insight into the molecular-level investigation of light-induced quantum processes in biological systems and nanostructured (bio)assemblies. Topics include DNA photostability and repair, photoactive proteins, biological and artificial light-harvesting systems, plasmonic nanostructures, and organic photovoltaic materials, whose common denominator is the key importance of ultrafast quantum effects at the border between the molecular scale and the nanoscale. The functionality and control of these systems have been under intense investigation in recent years in view of developing a detailed understanding of ultrafast nanoscale energy and charge transfer, as well as fostering novel technologies based on sustainable energy resources. Both experiment and theory have made big strides toward meeting the challenge of these truly complex systems. This book, thus, introduces the reader to cutting-edge developments in ultrafast nonlinear optical spectroscopies and the quantum dynamical simulation of the observed dynamics, including direct simulations of two-dimensional optical experiments. Taken together, these techniques attempt to elucidate whether the quantum coherent nature of ultrafast events enhances the efficiency of the relevant processes and where the quantum–classical boundary sets in, in these high-dimensional biological and material systems. The chapters contain well-illustrated accounts of the authors’ research work, including didactic introductory material, and address a multidisciplinary audience from chemistry, physics, biology, and materials sciences. The book is, therefore, a must-have for graduate- and postgraduate-level researchers who wish to learn about molecular nanoscience from a combined spectroscopic and theoretical viewpoint.
Book Synopsis Ultrafast Spin Dynamics at the Nanoscale by : Nanna Zhou Hagström
Download or read book Ultrafast Spin Dynamics at the Nanoscale written by Nanna Zhou Hagström and published by . This book was released on 2022 with total page pages. Available in PDF, EPUB and Kindle. Book excerpt:
Book Synopsis Theoretical Investigation on Light-driven Ultrafast Dynamics in Nanoscale by : Adrian Domínguez Castro
Download or read book Theoretical Investigation on Light-driven Ultrafast Dynamics in Nanoscale written by Adrian Domínguez Castro and published by . This book was released on 2022 with total page 0 pages. Available in PDF, EPUB and Kindle. Book excerpt: In this doctoral thesis, the three pillars of theoretical modeling such as interpretation, confirmation and prediction, have underlined the importance of simulations techniques in femtochemistry on the analysis and understanding of experimental data and the vaticination of photoinduced charge transfer. The significance and novelty of the studies presented is that due to the several challenges on the accurate description of the charge transfer processes involving the systems of interest, the benefits of the DFT and DFTB based calculations are highlighted. From the ground state description, the computation of X-ray absorption spectroscopy (XAS) and X-ray photoelectron spectroscopy (XPS) and the excited states studies applying the real-time Ehrenfest approach in the TDDFTB framework. This last method is a valuable tool for the study of large systems for new materials design with applications in photochemistry and nanophotonics. This work could be useful for the investigation on this topic in the near future.
Book Synopsis Ultrafast Dynamics In Molecules, Nanostructures And Interfaces - Selected Lectures Presented At Symposium On Ultrafast Dynamics Of The 7th International Conference On Materials For Advanced Technologies by : Guglielmo Lanzani
Download or read book Ultrafast Dynamics In Molecules, Nanostructures And Interfaces - Selected Lectures Presented At Symposium On Ultrafast Dynamics Of The 7th International Conference On Materials For Advanced Technologies written by Guglielmo Lanzani and published by World Scientific. This book was released on 2014-01-22 with total page 304 pages. Available in PDF, EPUB and Kindle. Book excerpt: Primary events in natural systems or devices occur on extremely short time scales, and yet determine in many cases the final performance or output. For this reason research in ultrafast science is of primary importance and impact in both fundamental research as well as its applications. This book reviews the advances in the field, addressing timely and open questions such as the role of quantum coherence in biology, the role of excess energy in electron injection at photovoltaic interfaces or the dynamics in quantum confined structures (e.g. multi carrier generation). The approach is that of a monograph, with a broad tutorial introduction and an overview of the recent results. This volume includes selected lectures presented at Symposium on Ultrafast Dynamics of the 7th International Conference on Materials for Advanced Technologies.
Book Synopsis Nanoscale Coherent Control. Ultrafast Dynamics of Single Molecules, Individual Light Harvesting Complexes and Discrete Nanoantennas at Room Temperature by : Daan Brinks
Download or read book Nanoscale Coherent Control. Ultrafast Dynamics of Single Molecules, Individual Light Harvesting Complexes and Discrete Nanoantennas at Room Temperature written by Daan Brinks and published by . This book was released on 2013 with total page 150 pages. Available in PDF, EPUB and Kindle. Book excerpt: Ultrafast pulses allow observation of molecular dynamics with femtosecond time resolution through pump probe experiments. However, averaging over an ensemble of molecules tends to wash out phase sensitive information, necessary to probe quantum effects, due to the intrinsic inhomogeneity in molecular conformations, orientations and interactions that lead to unique potential energy landscapes for each molecule. It is therefore important to go beyond the ensemble average when looking at quantum dynamics of organic systems at room temperature, and resolve the behaviour of specific molecules on an individual basis. In this thesis, we show the creation, manipulation and observation of ultrafast coherent effects in single molecules at room temperature, and resolve a certain measure of environmental influence on the specific dynamics of each molecule. Moreover, we apply this insight to investigate a functional light harvesting biosystem, and lay the basis for a technique that has the time and space resolution required to observe these systems in vivo. In chapter 1, we introduce the concepts and techniques the research in this thesis is built on. In chapter 2, we treat the possibility of controlling ultrafast pulses at the high-NA diffraction limit, and come to conclusions about the procedure to follow there that hold for all pulse-shaping experiments. We show in proof of principle experiments that we can control the ultrafast characteristics of optical pulses in nanometric excitation volumes. In chapters 3 and 4 we report the creation, detection and control of ultrafast quantum dynamics in single organic molecules at room temperature. We show that manipulation of superposition states is possible in these systems within a coherence dephasing time of ̃50 fs. This leads to the first observation of rabi-oscillations in room temperature single molecules, to ultrafast operation of an organic qubit, and to the creation of non-stationary superposition states (vibrational wavepackets). We probe the influence of the local environment on the composition and dynamics of these wavepackets and show we can optimize the state preparation protocol for each individual molecule in its own nanoenvironment, leading to high fidelity coherent control. In these chapters we lay out the proof of principle work of detecting the quantumdynamics of a complex system in interaction with its environment at room temperature. In chapter 5 we discuss application of these techniques to the investigation of long lived coherence in photosynthetic systems. We show that electronic coherence between different rings of the LH2 system persists to time scales of 100s of femtoseconds at room temperature. Moreover we show that the energy transfer pathways in LH2 adapt to environmentally induced changes in the molecule and that the nature of the transfer remains coherent for each pathway, providing strong evidence that coherent energy transfer is the optimum process for energy transfer in photosynthesis. Finally, in chapter 6 we take the technical development one step further and report on the creation of a framework based on plasmonic antennas that allows for control of the amplitude-phase characteristics in nanometric sized hotspot fields. We show for the first time that the ultrafast characteristics of plasmonic hotspots can directly be engineered through design of the plasmonic system and experimentally demonstrate two much-anticipated examples: a sub-diffraction resolution phase shaper and an ultrafast plasmonic switch for pump probe experiments. The results presented in this thesis form the first creation and observation of ultrafast coherent dynamics in individual molecular systems at room temperature. This is a necessary step to be able to do true quantum tomography in complex systems, resolve the influence of the environment on molecular dynamics, and investigate the physics that determines evolutionary optimization and functionality in biomolecules.
Book Synopsis Theory of Transport Properties of Semiconductor Nanostructures by : Eckehard Schöll
Download or read book Theory of Transport Properties of Semiconductor Nanostructures written by Eckehard Schöll and published by Springer Science & Business Media. This book was released on 2013-11-27 with total page 394 pages. Available in PDF, EPUB and Kindle. Book excerpt: Recent advances in the fabrication of semiconductors have created almost un limited possibilities to design structures on a nanometre scale with extraordinary electronic and optoelectronic properties. The theoretical understanding of elec trical transport in such nanostructures is of utmost importance for future device applications. This represents a challenging issue of today's basic research since it requires advanced theoretical techniques to cope with the quantum limit of charge transport, ultrafast carrier dynamics and strongly nonlinear high-field ef fects. This book, which appears in the electronic materials series, presents an over view of the theoretical background and recent developments in the theory of electrical transport in semiconductor nanostructures. It contains 11 chapters which are written by experts in their fields. Starting with a tutorial introduction to the subject in Chapter 1, it proceeds to present different approaches to transport theory. The semiclassical Boltzmann transport equation is in the centre of the next three chapters. Hydrodynamic moment equations (Chapter 2), Monte Carlo techniques (Chapter 3) and the cellular au tomaton approach (Chapter 4) are introduced and illustrated with applications to nanometre structures and device simulation. A full quantum-transport theory covering the Kubo formalism and nonequilibrium Green's functions (Chapter 5) as well as the density matrix theory (Chapter 6) is then presented.
Book Synopsis Imaging Nanoscale Morphology and Ultrafast Dynamics of Semiconducting Polymer Films with Time-resolved Photoemission Electron Microscopy by : Andreas Neff
Download or read book Imaging Nanoscale Morphology and Ultrafast Dynamics of Semiconducting Polymer Films with Time-resolved Photoemission Electron Microscopy written by Andreas Neff and published by . This book was released on 2017 with total page pages. Available in PDF, EPUB and Kindle. Book excerpt:
Book Synopsis Ultrafast Dynamics of Condensed Phase Systems by :
Download or read book Ultrafast Dynamics of Condensed Phase Systems written by and published by . This book was released on 2000 with total page 0 pages. Available in PDF, EPUB and Kindle. Book excerpt: In this final report, we describe the results of our ONR-funded research project in theoretical and computational chemistry. We briefly review our ONR-supported work in the following areas: (1) Development of methodology for simulating nonadiabatic dynamics in molecular systems. (2) A proposal for a new type of direct spectroscopy of ultrafast many-body bath dynamics, called nanoscale shock wave spectroscopy, and the results of molecular dynamics simulations describing its theoretical implementation.
Book Synopsis Ultrafast Dynamics Driven by Intense Light Pulses by : Markus Kitzler
Download or read book Ultrafast Dynamics Driven by Intense Light Pulses written by Markus Kitzler and published by Springer. This book was released on 2015-07-24 with total page 385 pages. Available in PDF, EPUB and Kindle. Book excerpt: This book documents the recent vivid developments in the research field of ultrashort intense light pulses for probing and controlling ultrafast dynamics. The recent fascinating results in studying and controlling ultrafast dynamics in ever more complicated systems such as (bio-)molecules and structures of meso- to macroscopic sizes on ever shorter time-scales are presented. The book is written by some of the most eminent experimental and theoretical experts in the field. It covers the new groundbreaking research directions that were opened by the availability of new light sources such as fully controlled intense laser fields with durations down to a single oscillation cycle, short-wavelength laser-driven attosecond pulses and intense X-ray pulses from the upcoming free electron lasers. These light sources allowed the investigation of dynamics in atoms, molecules, clusters, on surfaces and very recently also in nanostructures and solids in new regimes of parameters which, in turn, led to the identification of completely new dynamics and methods for controlling it. Example topics covered by this book include the study of ultrafast processes in large molecules using attosecond pulses, control of ultrafast electron dynamics in solids with shaped femtosecond laser pulses, light-driven ultrafast plasmonic processes on surfaces and in nanostructures as well as research on atomic and molecular systems under intense X-ray radiation. This book is equally helpful for people who would like to step into this field (e.g. young researchers), for whom it provides a broad introduction, as well as for already experienced researchers who may enjoy the exhaustive discussion that covers the research on essentially all currently studied objects and with all available ultrafast pulse sources.
Book Synopsis Nanoscale Materials by : Luis M. Liz-Marzán
Download or read book Nanoscale Materials written by Luis M. Liz-Marzán and published by Springer Science & Business Media. This book was released on 2007-05-08 with total page 506 pages. Available in PDF, EPUB and Kindle. Book excerpt: Organized nanoassemblies of inorganic nanoparticles and organic molecules are building blocks of nanodevices, whether they are designed to perform molecular level computing, sense the environment or improve the catalytic properties of a material. The key to creation of these hybrid nanostructures lies in understanding the chemistry at a fundamental level. This book serves as a reference book for researchers by providing fundamental understanding of many nanoscopic materials.
Book Synopsis Nanoscale Photonic Imaging by : Tim Salditt
Download or read book Nanoscale Photonic Imaging written by Tim Salditt and published by Springer Nature. This book was released on 2020-06-09 with total page 634 pages. Available in PDF, EPUB and Kindle. Book excerpt: This open access book, edited and authored by a team of world-leading researchers, provides a broad overview of advanced photonic methods for nanoscale visualization, as well as describing a range of fascinating in-depth studies. Introductory chapters cover the most relevant physics and basic methods that young researchers need to master in order to work effectively in the field of nanoscale photonic imaging, from physical first principles, to instrumentation, to mathematical foundations of imaging and data analysis. Subsequent chapters demonstrate how these cutting edge methods are applied to a variety of systems, including complex fluids and biomolecular systems, for visualizing their structure and dynamics, in space and on timescales extending over many orders of magnitude down to the femtosecond range. Progress in nanoscale photonic imaging in Göttingen has been the sum total of more than a decade of work by a wide range of scientists and mathematicians across disciplines, working together in a vibrant collaboration of a kind rarely matched. This volume presents the highlights of their research achievements and serves as a record of the unique and remarkable constellation of contributors, as well as looking ahead at the future prospects in this field. It will serve not only as a useful reference for experienced researchers but also as a valuable point of entry for newcomers.
Book Synopsis Ultrafast Spectroscopy by : Joel Yuen-Zhou
Download or read book Ultrafast Spectroscopy written by Joel Yuen-Zhou and published by Iop Expanding Physics. This book was released on 2014 with total page 0 pages. Available in PDF, EPUB and Kindle. Book excerpt: The goal of this book is to provide a simple and conceptually intuitive introduction to nonlinear spectroscopy via the formalism of quantum processes and wavepacket dynamics.
Book Synopsis Size Dependent Ultrafast Ionization Dynamics of Nanoscale Samples in Intense Femtosecond X-ray Free Electron Laser Pulses by :
Download or read book Size Dependent Ultrafast Ionization Dynamics of Nanoscale Samples in Intense Femtosecond X-ray Free Electron Laser Pulses written by and published by . This book was released on 2012 with total page 112 pages. Available in PDF, EPUB and Kindle. Book excerpt:
Book Synopsis Experimental Study of Electron and Phonon Dynamics in Nanoscale Materials by Ultrafast Laser Time-domain Spectroscopy by : Xiaohan Shen
Download or read book Experimental Study of Electron and Phonon Dynamics in Nanoscale Materials by Ultrafast Laser Time-domain Spectroscopy written by Xiaohan Shen and published by . This book was released on 2017 with total page 310 pages. Available in PDF, EPUB and Kindle. Book excerpt:
Book Synopsis Development of High-brightness Ultrafast Electron Microscope for Studying Nanoscale Dynamics Associated with Strongly Correlated Materials by : Zhensheng Tao
Download or read book Development of High-brightness Ultrafast Electron Microscope for Studying Nanoscale Dynamics Associated with Strongly Correlated Materials written by Zhensheng Tao and published by . This book was released on 2014 with total page 300 pages. Available in PDF, EPUB and Kindle. Book excerpt:
Author :Takayoshi Kobayashi Publisher :Springer Science & Business Media ISBN 13 :9783540241102 Total Pages :954 pages Book Rating :4.2/5 (411 download)
Book Synopsis Ultrafast Phenomena XIV by : Takayoshi Kobayashi
Download or read book Ultrafast Phenomena XIV written by Takayoshi Kobayashi and published by Springer Science & Business Media. This book was released on 2005 with total page 954 pages. Available in PDF, EPUB and Kindle. Book excerpt: Ultrafast Phenomena XIV presents the latest advances in ultrafast science, including ultrafast laser and measurement technology as well as studies of ultrafast phenomena. Pico-, femto-, and atosecond processes relevant in physics, chemistry, biology and engineering are presented. Ultrafast technology is now having a profound impact within a wide range of applications, among them imaging, material diagnostics, and transformation and high-speed optoelectronics. This book summarizes results presented at the 14th Ultrafast Phenomena Conference and reviews the state of the art in this important and rapidly advancing field.
