Experimental Study of Electron and Phonon Dynamics in Nanoscale Materials by Ultrafast Laser Time-domain Spectroscopy

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ISBN 13 :
Total Pages : 310 pages
Book Rating : 4.:/5 (115 download)

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Book Synopsis Experimental Study of Electron and Phonon Dynamics in Nanoscale Materials by Ultrafast Laser Time-domain Spectroscopy by : Xiaohan Shen

Download or read book Experimental Study of Electron and Phonon Dynamics in Nanoscale Materials by Ultrafast Laser Time-domain Spectroscopy written by Xiaohan Shen and published by . This book was released on 2017 with total page 310 pages. Available in PDF, EPUB and Kindle. Book excerpt:

Length-Scale Dependent Phonon Interactions

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Publisher : Springer Science & Business Media
ISBN 13 : 1461486513
Total Pages : 304 pages
Book Rating : 4.4/5 (614 download)

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Book Synopsis Length-Scale Dependent Phonon Interactions by : Subhash L. Shindé

Download or read book Length-Scale Dependent Phonon Interactions written by Subhash L. Shindé and published by Springer Science & Business Media. This book was released on 2013-10-29 with total page 304 pages. Available in PDF, EPUB and Kindle. Book excerpt: This book presents a comprehensive description of phonons and their interactions in systems with different dimensions and length scales. Internationally-recognized leaders describe theories and measurements of phonon interactions in relation to the design of materials with exotic properties such as metamaterials, nano-mechanical systems, next-generation electronic, photonic, and acoustic devices, energy harvesting, optical information storage, and applications of phonon lasers in a variety of fields. The emergence of techniques for control of semiconductor properties and geometry has enabled engineers to design structures in which functionality is derived from controlling electron behavior. As manufacturing techniques have greatly expanded the list of available materials and the range of attainable length scales, similar opportunities now exist for designing devices whose functionality is derived from controlling phonon behavior. However, progress in this area is hampered by gaps in our knowledge of phonon transport across and along arbitrary interfaces, the scattering of phonons with crystal defects, interface roughness and mass-mixing, delocalized electrons/collective electronic excitations, and solid acoustic vibrations when these occur in structures with small physical dimensions. This book provides a comprehensive description of phonons and their interactions in systems with different dimensions and length scales. Theories and measurements of phonon interactions are described in relation to the design of materials with exotic properties such as metamaterials, nano-mechanical systems, next-generation electronic, photonic, and acoustic devices, energy harvesting, optical information storage, and applications of phonon lasers in a variety of fields.

Time-resolved THz Studies of Carrier Dynamics in Semiconductors, Superconductors, and Strongly-correlated Electron Materials

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ISBN 13 :
Total Pages : pages
Book Rating : 4.:/5 (893 download)

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Book Synopsis Time-resolved THz Studies of Carrier Dynamics in Semiconductors, Superconductors, and Strongly-correlated Electron Materials by :

Download or read book Time-resolved THz Studies of Carrier Dynamics in Semiconductors, Superconductors, and Strongly-correlated Electron Materials written by and published by . This book was released on 2006 with total page pages. Available in PDF, EPUB and Kindle. Book excerpt: Perhaps the most important aspect of contemporary condensed matter physics involves understanding strong Coulomb interactions between the large number of electrons in a solid. Electronic correlations lead to the emergence of new system properties, such as metal-insulator transitions, superconductivity, magneto-resistance, Bose-Einstein condensation, the formation of excitonic gases, or the integer and fractional Quantum Hall effects. The discovery of high-Tc superconductivity in particular was a watershed event, leading to dramatic experimental and theoretical advances in the field of correlated-electron systems. Such materials often exhibit competition between the charge, lattice, spin, and orbital degrees of freedom, whose cause-effect relationships are difficult to ascertain. Experimental insight into the properties of solids is traditionally obtained by time-averaged probes, which measure e.g., linear optical spectra, electrical conduction properties, or the occupied band structure in thermal equilibrium. Many novel physical properties arise from excitations out of the ground state into energetically higher states by thermal, optical, or electrical means. This leads to fundamental interactions between the system's constituents, such as electron-phonon and electron-electron interactions, which occur on ultrafast timescales. While these interactions underlie the physical properties of solids, they are often only indirectly inferred from time-averaged measurements. Time-resolved spectroscopy, consequently, is playing an ever increasing role to provide insight into light-matter interaction, microscopic processes, or cause-effect relationships that determine the physics of complex materials. In the past, experiments using visible and near-infrared femtosecond pulses have been extensively employed, e.g. to follow relaxation and dephasing processes in metals and semiconductors. However, many basic excitations in strongly-correlated electron systems and nanoscale materials occur at lower energies. The terahertz (THz) regime is particularly rich in such fundamental resonances. This includes ubiquitous lattice vibrations and low-energy collective oscillations of conduction charges. In nanoscale materials, band structure quantization also yields novel infrared and THz transitions, including intersubband absorption in quantum wells. The formation of excitons in turn leads to low-energy excitations analogous to inter-level transitions in atoms. In transition-metal oxides, fundamental excitation gaps arise from charge pairing into superconducting condensates and other correlated states. This motivates the use of ultrafast THz spectroscopy as a powerful tool to study light-matter interactions and microscopic processes in nanoscale and correlated-electron materials. A distinct advantage of coherent THz pulses is that the amplitude and phase of the electric field can be measured directly, as the THz fields are coherent with the fs pulses from which they are generated. Using THz time-domain spectroscopy (THz-TDS), both the real and imaginary parts of the response functions (such as the dielectric function) are obtained directly without the need for Kramers?Kronig transforms. The THz response can also be expressed in terms of absorption and refractive index, or as the optical conductivity. The optical conductivity describes the current response of a many-body system to an electric field, an ideal tool to study conducting systems. A second important advantage is the ultrafast time resolution that results from the short temporal duration of the THz time-domain sources. In particular, optical-pump THz-probe spectroscopy enables a delicate probe of the transient THz conductivity after optical photoexcitation. These experiments can provide insight into quasiparticle interactions, phase transitions, or nonequilibrium dynamics. In this chapter we will provide many such examples. Since THz spectroscopy of solids is a quickly expanding field.

Quantum Phononics

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Publisher : Springer
ISBN 13 : 3030119246
Total Pages : 142 pages
Book Rating : 4.0/5 (31 download)

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Book Synopsis Quantum Phononics by : Kazutaka Nakamura

Download or read book Quantum Phononics written by Kazutaka Nakamura and published by Springer. This book was released on 2019-02-20 with total page 142 pages. Available in PDF, EPUB and Kindle. Book excerpt: This book presents quantum phononics as an exciting new field of research, and introduces readers to the quantum nature of phonons and their application to quantum technologies. Both the theory of and recent experiments in “quantum phononics,” involving e.g. coherent phonons, phonon squeezing, coherent control, and phonon quantum technologies, are presented. The theoretical background of the generation and detection of phonons is described in a way that will be easy to understand for graduate students and experimental scientists who are newcomers to the field. Moreover, the book focuses on coherent phonons produced by ultrafast laser pulses, which can be used for the coherent control of atomic motions in solids and phase transformation. The laser-matter interaction is treated using a density matrix formalism of the time-dependent Schröedinger equation. In addition, the third-order nonlinear optical response of condensed matter is also described.

A Study of Electron and Phonon Dynamics by Broadband Two-dimensional THz Time-domain Spectroscopy

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ISBN 13 :
Total Pages : 198 pages
Book Rating : 4.:/5 (115 download)

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Book Synopsis A Study of Electron and Phonon Dynamics by Broadband Two-dimensional THz Time-domain Spectroscopy by : Zhengping Fu

Download or read book A Study of Electron and Phonon Dynamics by Broadband Two-dimensional THz Time-domain Spectroscopy written by Zhengping Fu and published by . This book was released on 2016 with total page 198 pages. Available in PDF, EPUB and Kindle. Book excerpt:

Handbook of Laser Technology and Applications

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Publisher : CRC Press
ISBN 13 : 1315310848
Total Pages : 359 pages
Book Rating : 4.3/5 (153 download)

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Book Synopsis Handbook of Laser Technology and Applications by : Chunlei Guo

Download or read book Handbook of Laser Technology and Applications written by Chunlei Guo and published by CRC Press. This book was released on 2021-06-23 with total page 359 pages. Available in PDF, EPUB and Kindle. Book excerpt: This comprehensive handbook gives a fully updated guide to lasers and laser technologies, including the complete range of their technical applications. This third volume covers modern applications in engineering and technology, including all new and updated case studies spanning telecommunications and data storage to medicine, optical measurement, defense and security, nanomaterials processing and characterization. Key Features: • Offers a complete update of the original, bestselling work, including many brand-new chapters. • Deepens the introduction to fundamentals, from laser design and fabrication to host matrices for solid-state lasers, energy level diagrams, hosting materials, dopant energy levels, and lasers based on nonlinear effects. • Covers new laser types, including quantum cascade lasers, silicon-based lasers, titanium sapphire lasers, terahertz lasers, bismuth-doped fiber lasers, and diode-pumped alkali lasers. • Discusses the latest applications, e.g., lasers in microscopy, high-speed imaging, attosecond metrology, 3D printing, optical atomic clocks, time-resolved spectroscopy, polarization and profile measurements, pulse measurements, and laser-induced fluorescence detection. • Adds new sections on laser materials processing, laser spectroscopy, lasers in imaging, lasers in environmental sciences, and lasers in communications. This handbook is the ideal companion for scientists, engineers, and students working with lasers, including those in optics, electrical engineering, physics, chemistry, biomedicine, and other relevant areas.

Encyclopedia of Modern Optics

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Publisher : Academic Press
ISBN 13 : 0128149825
Total Pages : 2253 pages
Book Rating : 4.1/5 (281 download)

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Book Synopsis Encyclopedia of Modern Optics by : Bob D. Guenther

Download or read book Encyclopedia of Modern Optics written by Bob D. Guenther and published by Academic Press. This book was released on 2018-02-14 with total page 2253 pages. Available in PDF, EPUB and Kindle. Book excerpt: The Encyclopedia of Modern Optics, Second Edition, Five Volume Set provides a wide-ranging overview of the field, comprising authoritative reference articles for undergraduate and postgraduate students and those researching outside their area of expertise. Topics covered include classical and quantum optics, lasers, optical fibers and optical fiber systems, optical materials and light-emitting diodes (LEDs). Articles cover all subfields of optical physics and engineering, such as electro-optical design of modulators and detectors. This update contains contributions from international experts who discuss topics such as nano-photonics and plasmonics, optical interconnects, photonic crystals and 2D materials, such as graphene or holy fibers. Other topics of note include solar energy, high efficiency LED’s and their use in illumination, orbital angular momentum, quantum optics and information, metamaterials and transformation optics, high power fiber and UV fiber lasers, random lasers and bio-imaging. Addresses recent developments in the field and integrates concepts from fundamental physics with applications for manufacturing and engineering/design Provides a broad and interdisciplinary coverage of specialist areas Ensures that the material is appropriate for new researchers and those working in a new sub-field, as well as those in industry Thematically arranged and alphabetically indexed, with cross-references added to facilitate ease-of-use

Electron-phonon Dynamics And Jahn-teller Effect - Proceedings Of The Xiv International Symposium

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Publisher : World Scientific
ISBN 13 : 9814543721
Total Pages : 412 pages
Book Rating : 4.8/5 (145 download)

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Book Synopsis Electron-phonon Dynamics And Jahn-teller Effect - Proceedings Of The Xiv International Symposium by : N Terzi

Download or read book Electron-phonon Dynamics And Jahn-teller Effect - Proceedings Of The Xiv International Symposium written by N Terzi and published by World Scientific. This book was released on 1999-08-31 with total page 412 pages. Available in PDF, EPUB and Kindle. Book excerpt: The Jahn-Teller effect is a consequence of the electron-phonon coupling in high symmetry systems. Its influence covers a wide range of physical and chemical properties and systems. As the biannual Jahn-Teller symposia bring together experimental and theoretical physicists and chemists from all over the world, this proceedings volume reports the latest scientific news on the effect.The contents of the volume range from the general aspects to some special topics, such as ultrafast processes, fullerenes, point defects, cooperative phenomena, HTSC and oxide properties. Some contributions are dedicated to the memory of Mary O'Brien, a globally honored specialist in the theory of the Jahn-Teller effect. Throughout personal reminiscences of O'Brien's enormous contributions to the subject, the recent history of the effect is summarized.

The Physics of Phonons

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Publisher : CRC Press
ISBN 13 : 1000686981
Total Pages : 674 pages
Book Rating : 4.0/5 (6 download)

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Book Synopsis The Physics of Phonons by : Gyaneshwar P. Srivastava

Download or read book The Physics of Phonons written by Gyaneshwar P. Srivastava and published by CRC Press. This book was released on 2022-09-28 with total page 674 pages. Available in PDF, EPUB and Kindle. Book excerpt: This fully updated second edition of The Physics of Phonons remains the most comprehensive theoretical discussion devoted to the study of phonons, a major area of condensed matter physics. It contains exciting new sections on phonon-related properties of solid surfaces, atomically thin materials (such as graphene and monolayer transition metal chalcogenides), in addition to nano- structures and nanocomposites, thermoelectric nanomaterials, and topological nanomaterials, with an entirely new chapter dedicated to topological nanophononics and chiralphononics. Although primarily theoretical in approach, the author refers to experimental results wherever possible, ensuring an ideal book for both experimental and theoretical researchers. The author begins with an introduction to crystal symmetry and continues with a discussion of lattice dynamics in the harmonic approximation, including the traditional phenomenological approach and the more recent ab initio approach, detailed for the first time in this book. A discussion of anharmonicity is followed by the theory of lattice thermal conductivity, presented at a level far beyond that available in any other book. The chapter on phonon interactions is likewise more comprehensive than any similar discussion elsewhere. The sections on phonons in superlattices, impure and mixed crystals, quasicrystals, phonon spectroscopy, Kapitza resistance, and quantum evaporation also contain material appearing in book form for the first time. The book is complemented by numerous diagrams that aid understanding and is comprehensively referenced for further study. With its unprecedented wide coverage of the field, The Physics of Phonons is an indispensable guide for advanced undergraduates, postgraduates, and researchers working in condensed matter physics and materials science. Features Fully updated throughout, with exciting new coverage on graphene, nanostructures and nanocomposites, thermoelectric nanomaterials, and topological nanomaterials. Authored by an authority on phonons. Interdisciplinary, with broad applications through condensed matter physics, nanoscience, and materials science. --

Frontiers in Optical Methods

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Publisher : Springer
ISBN 13 : 3642405940
Total Pages : 233 pages
Book Rating : 4.6/5 (424 download)

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Book Synopsis Frontiers in Optical Methods by : Ken-ichi Shudo

Download or read book Frontiers in Optical Methods written by Ken-ichi Shudo and published by Springer. This book was released on 2013-12-04 with total page 233 pages. Available in PDF, EPUB and Kindle. Book excerpt: This collection of reviews by leading Japanese researchers covers topics like ultrafast optical responses, terahertz and phonon studies, super-sensitive surface and high-pressure spectroscopy, combination of visible and x-ray photonics. Several related areas at the cutting edge of measurement technology and materials science are included. This book is partly based on well-cited review articles in the Japanese language in special volumes of the Journal of the Vacuum Society of Japan.

Femtosecond Laser-Matter Interaction

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Publisher : CRC Press
ISBN 13 : 9814241814
Total Pages : 370 pages
Book Rating : 4.8/5 (142 download)

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Book Synopsis Femtosecond Laser-Matter Interaction by : Eugene G. Gamaly

Download or read book Femtosecond Laser-Matter Interaction written by Eugene G. Gamaly and published by CRC Press. This book was released on 2011-10-06 with total page 370 pages. Available in PDF, EPUB and Kindle. Book excerpt: This is the first comprehensive treatment of the interaction of femtosecond laser pulses with solids at nonrelativistic intensity. It connects phenomena from the subtle atomic motion on the nanoscale to the generation of extreme pressure and temperature in the interaction zone confined inside a solid. The femtosecond laser-matter interaction has already found numerous applications in industry, medicine, and materials science. However, there is no consensus on the interpretation of related phenomena. With mathematics kept to a minimum, this is a highly engaging and readable treatment for students and researchers in science and engineering. The book avoids complex mathematical formulae, and hence the content is accessible to nontechnical readers. Useful summaries after each chapter provide compressed information for quick estimates of major parameters in planned or performed experiments. The book connects the basic physics of femtosecond laser-solid interactions to a broad range of applications. Throught the text, basic assumptions are derived from the first principles, and new results and ideas are presented. From such analyses, a qualitative and predictive framework for the field emerges, the impact of which on applications is also discussed.

Electron-phonon Interactions in Low-dimensional Structures

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ISBN 13 : 9780198507321
Total Pages : 302 pages
Book Rating : 4.5/5 (73 download)

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Book Synopsis Electron-phonon Interactions in Low-dimensional Structures by : Lawrence John Challis

Download or read book Electron-phonon Interactions in Low-dimensional Structures written by Lawrence John Challis and published by . This book was released on 2003 with total page 302 pages. Available in PDF, EPUB and Kindle. Book excerpt: The study of electrons and holes confined to two, one and even zero dimensions has uncovered a rich variety of new physics and applications. This book describes the interaction between these confined carriers and the optic and acoustic phonons within and around the confined regions. Phonons provide the principal channel of energy transfer between the carriers and their surroundings and also the main restriction to their room temperature mobility. But they have many other roles; they provide, for example, an essential feature of the operation of the quantum cascade laser. Since their momenta at relevant energies are well matched to those of electrons, they can also be used to probe electronic properties such as the confinement width of 2D electron gases and the dispersion curve of quasiparticles in the fractional quantum Hall effect. The book describes both the physics of the electron-phonon interaction in the different confined systems and the experimental and theoretical techniques that have been used in its investigation. The experimental methods include optical and transport techniques as well as techniques in which phonons are used as the experimental probe. The aim of the book is to provide an up to date review of the physics and its significance in device performance. It is also written to be explanatory and accessible to graduate students and others new to the field.

Optical Spectroscopy at the Nanoscale

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Publisher :
ISBN 13 :
Total Pages : 85 pages
Book Rating : 4.:/5 (18 download)

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Book Synopsis Optical Spectroscopy at the Nanoscale by : Xiaoping Hong

Download or read book Optical Spectroscopy at the Nanoscale written by Xiaoping Hong and published by . This book was released on 2014 with total page 85 pages. Available in PDF, EPUB and Kindle. Book excerpt: Recent advances in material science and fabrication techniques enabled development of nanoscale applications and devices with superior performances and high degree of integration. Exotic physics also emerges at nanoscale where confinement of electrons and phonons leads to drastically different behavior from those in the bulk materials. It is therefore rewarding and interesting to investigate and understand material properties at the nanoscale. Optical spectroscopy, one of the most versatile techniques for studying material properties and light-matter interactions, can provide new insights into the nanomaterials. In this thesis, I explore advanced laser spectroscopic techniques to probe a variety of different nanoscale phenomena. A powerful tool in nanoscience and engineering is scanning tunneling microscopy (STM). Its capability in atomic resolution imaging and spectroscopy unveiled the mystical quantum world of atoms and molecules. However identification of molecular species under investigation is one of the limiting functionalities of the STM. To address this need, we take advantage of the molecular `fingerprints' - vibrational spectroscopy, by combining an infrared light sources with scanning tunneling microscopy. In order to map out sharp molecular resonances, an infrared continuous wave broadly tunable optical parametric oscillator was developed with mode-hop free fine tuning capabilities. We then combine this laser with STM by shooting the beam onto the STM substrate with sub-monolayer diamondoids deposition. Thermal expansion of the substrate is detected by the ultrasensitive tunneling current when infrared frequency is tuned across the molecular vibrational range. Molecular vibrational spectroscopy could be obtained by recording the thermal expansion as a function of the excitation wavelength. Another interesting field of the nanoscience is carbon nanotube, an ideal model of one dimensional physics and applications. Due to the small light absorption with nanometer size, individual carbon nanotube is not visible under any conventional microscopy and characterization of individual nanotube becomes a focused research interest. Although electron microscopies and optical spectroscopies are developed previously to study carbon nanotubes, none of them permitted versatile imaging and spectroscopy of individual nanotube in a non-invasive, high throughput and ambient way. In this thesis a new polarization-based optical microscopy and spectroscopy is developed with exceedingly better contrast for one dimensional nano-materials and capability of individual carbon nanotube imaging and spectroscopy. This development provides a reliable way to measure the absolute absorption cross-section of individual chirality-defined carbon nanotubes. It also enables fast profiling for growth optimization and in situ characterization for functioning carbon nanotube devices. Two dimensional systems constitute another important family of nanomaterials, ranging from semi-metal (graphene), semiconductors (transition metal dichalcogenides) to insulators (h-BN). Despite of their scientific significance, they present a complete set of 2D building blocks for two dimensional electronics and optoelectronics. Heterostructures purely made of 2D thin films hold great promises due to functionality, scalability and ultrathin nature. Understanding the properties of the coupled heterolayers will be important and intriguing for these applications. With the advanced ultrafast laser spectroscopy, we study the dynamics of charge transfer process in two dimensional atomically thin semiconductors heterostructures. An extremely efficient charge transfer process is identified in atomically thin MoS2/WS2 system, which is expected to form a type-II heterojunction. Our discovery would greatly facilitate further studies of 2D materials as a photovoltaic device.

Ultrafast Investigations of Exciton Dynamics in 0D and 2D Hybrid Semiconductor Nanomaterials

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Publisher :
ISBN 13 :
Total Pages : 0 pages
Book Rating : 4.:/5 (139 download)

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Book Synopsis Ultrafast Investigations of Exciton Dynamics in 0D and 2D Hybrid Semiconductor Nanomaterials by : Eric R. Powers

Download or read book Ultrafast Investigations of Exciton Dynamics in 0D and 2D Hybrid Semiconductor Nanomaterials written by Eric R. Powers and published by . This book was released on 2023 with total page 0 pages. Available in PDF, EPUB and Kindle. Book excerpt: The development of hybrid organic-inorganic semiconductor nanomaterials represents a major advance towards highly tunable and efficient optoelectronic devices. These materials are comprised of multiple chemical constituents arranged in nanoscale geometries, and they exhibit emergent properties such as quantum confinement and enhanced Coulombic interactions. Photoactive nanomaterials have potential applications in lighting, solar, lasing, and quantum information. However, their complex chemistry and nanometer-scale dimensionality present a barrier to understanding and controlling their structure-function relationships. In this thesis, I utilize ultrafast pump-probe spectroscopy to study the fundamental properties of hybrid semiconductor nanomaterials. This technique allows the electronic and vibrational dynamics of these materials to be investigated with femtosecond time resolution, providing new insights into their underlying physics. I first employ impulsive vibrational spectroscopy to study exciton-phonon interactions in silver phenyl selenolate (AgSePh), a recently discovered hybrid 2D semiconductor. Combining this time-domain Raman technique with frequency-domain non-resonant Raman scattering, I measure the vibrational landscape of the system and identify a subset of vibrational modes that couple strongly to excitonic transitions. Density functional theory calculations are then utilized to pinpoint specific atomic displacements which couple to the excitonic transition. An investigation of temperature-dependent photoluminescence reveals the connection between atomic scale dynamics and macroscopic properties, showing the 99 cm−1 mode strongly impacts emission frequency and linewidth in AgSePh. Finally, temperature-dependent impulsive vibrational spectroscopy is employed to probe vibrational anharmonicity in this material. These findings provide a roadmap for controlling exciton-phonon coupling in hybrid organic-inorganic semiconductors. Next, I study charging and neutralization processes in lead halide perovskite nanocrystals (quantum dots) with transient absorption spectroscopy. A temperature-dependent study of CsPbBr3 nanocrystals reveals that charging occurs in a significant fraction of photoexcited nanocrystals (>10%), which then exhibit a microsecond neutralization lifetime at cryogenic temperatures. The temperature-dependent dynamics are modeled to extract a ~100 meV energy barrier to re-neutralization. Additionally, photocharging shows a sublinear fluence dependence, excluding Auger recombination as the initiator of this process, in contrast with traditional nanocrystal systems. These results help illuminate the underlying mechanism of charging in perovskite nanocrystals, guiding future synthetic advances to improve nanocrystal performance in lighting and quantum information applications.

Spectroscopy of Nonequilibrium Electrons and Phonons

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Publisher :
ISBN 13 :
Total Pages : 520 pages
Book Rating : 4.X/5 (2 download)

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Book Synopsis Spectroscopy of Nonequilibrium Electrons and Phonons by : Charles V. Shank

Download or read book Spectroscopy of Nonequilibrium Electrons and Phonons written by Charles V. Shank and published by . This book was released on 1992 with total page 520 pages. Available in PDF, EPUB and Kindle. Book excerpt: The physics of nonequilibrium electrons and phonons in semiconductors is an important branch of fundamental physics that has many practical applications, especially in the development of ultrafast and ultrasmall semiconductor devices. This volume is devoted to different trends in the field which are presently at the forefront of research. Special attention is paid to the ultrafast relaxation processes in bulk semiconductors and two-dimensional semiconductor structures, and to their study by different spectroscopic methods, both pulsed and steady-state. and the relaxation kinetics of hot carriers and phonons are considered under various conditions such as temperature, doping and pumping intensity by leading experts in the field.

Femtosecond Time-resolved Spectroscopy of Coherent Oscillations in Nanomaterials

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ISBN 13 :
Total Pages : pages
Book Rating : 4.:/5 (61 download)

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Book Synopsis Femtosecond Time-resolved Spectroscopy of Coherent Oscillations in Nanomaterials by : Serguei Nikolaevich Jerebtsov

Download or read book Femtosecond Time-resolved Spectroscopy of Coherent Oscillations in Nanomaterials written by Serguei Nikolaevich Jerebtsov and published by . This book was released on 2010 with total page pages. Available in PDF, EPUB and Kindle. Book excerpt: The interaction of laser radiation with a material can excite coherent lattice vibration. The observation of such periodic motion of the atoms in the lattice provides information on the properties of the material. In the present work a femtosecond pump-probe technique was applied for studies of acoustic vibrations in nanoparticles and nanowires, and coherent optical phonons in thin films. The elastic properties of spherical Ag nanoparticles and Ag and Bi nanowires were studied in a dual-color femtosecond pump-probe experiment. The results of the period determinations of the acoustic vibrations, obtained from the time-domain measurements with low intensity pump pulses, together with the information about the size of the particles, were used to determine the elastic constants of the materials. Also changes in the measured acoustical response of the Ag nanowires under high intensity laser excitation were studied. In addition the coherent optical phonon excitation in a Bi film was studied in a femtosecond pump-probe experiment. A red-shift of the phonon frequency at the high photoexcitation density was observed. To separate the effect of the lattice softening and the lattice anharmonicity the excitation with two pump pulses was employed. Numerical simulations, which took into account the evolution of the spatial inhomogeneity of the excitation density, were carried out and compared to the experimental results.

Applied Spectroscopy and the Science of Nanomaterials

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Publisher : Springer
ISBN 13 : 9812872426
Total Pages : 284 pages
Book Rating : 4.8/5 (128 download)

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Book Synopsis Applied Spectroscopy and the Science of Nanomaterials by : Prabhakar Misra

Download or read book Applied Spectroscopy and the Science of Nanomaterials written by Prabhakar Misra and published by Springer. This book was released on 2014-10-21 with total page 284 pages. Available in PDF, EPUB and Kindle. Book excerpt: This book focuses on several areas of intense topical interest related to applied spectroscopy and the science of nanomaterials. The eleven chapters in the book cover the following areas of interest relating to applied spectroscopy and nanoscience: · Raman spectroscopic characterization, modeling and simulation studies of carbon nanotubes, · Characterization of plasma discharges using laser optogalvanic spectroscopy, · Fluorescence anisotropy in understanding protein conformational disorder and aggregation, · Nuclear magnetic resonance spectroscopy in nanomedicine, · Calculation of Van der Waals interactions at the nanoscale, · Theory and simulation associated with adsorption of gases in nanomaterials, · Atom-precise metal nanoclusters, · Plasmonic properties of metallic nanostructures, two-dimensional materials, and their composites, · Applications of graphene in optoelectronic devices and transistors, · Role of graphene in organic photovoltaic device technology, · Applications of nanomaterials in nanomedicine.