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Carbonaceous Aerosol Study Using Advanced Particle Instrumentation
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Book Synopsis Carbonaceous Aerosol Study Using Advanced Particle Instrumentation by : Li Qi
Download or read book Carbonaceous Aerosol Study Using Advanced Particle Instrumentation written by Li Qi and published by . This book was released on 2010 with total page 250 pages. Available in PDF, EPUB and Kindle. Book excerpt: A study of the evolution of carbonaceous aerosol in the atmosphere was conducted with special focus on primary biomass burning and secondary organic aerosol (SOA) processing. The work is broken down into two major components: the organic aerosol mass released from biomass burning and the evolution of SOA with special emphasis on formation routes. The biomass burning work explored the evolution of organic aerosol emissions as a function of modified combustion efficiency with correlations drawn between levoglucosan emissions and wood-type, combustion type (flaming, mixed, smoldering) using high resolution aerosol mass spectrometry. The SOA work includes insights into the mechanism for SOA formation from aromatics including the impacts of temperature and particle-aging. This work conclusively demonstrates that gas-particle partitioning theory combined with enthalpies of formation are insufficient to model the formation of SOA as a function of time; that the presence of secondary reactions, in both the particle and gas-phase continue to evolve the aerosol beyond that typically simulated in environmental chambers; and that current mechanisms for SOA formation from aromatics fail to explain isotopically labeled experiments while conclusively ruling out the importance of organic nitrate products.
Book Synopsis Laboratory Experiments and Instrument Intercomparison Studies of Carbonaceous Aerosol Particles by :
Download or read book Laboratory Experiments and Instrument Intercomparison Studies of Carbonaceous Aerosol Particles written by and published by . This book was released on 2015 with total page 13 pages. Available in PDF, EPUB and Kindle. Book excerpt: Aerosols containing black carbon (and some specific types of organic particulate matter) directly absorb incoming light, heating the atmosphere. In addition, all aerosol particles backscatter solar light, leading to a net-cooling effect. Indirect effects involve hydrophilic aerosols, which serve as cloud condensation nuclei (CCN) that affect cloud cover and cloud stability, impacting both atmospheric radiation balance and precipitation patterns. At night, all clouds produce local warming, but overall clouds exert a net-cooling effect on the Earth. The effect of aerosol radiative forcing on climate may be as large as that of the greenhouse gases, but predominantly opposite in sign and much more uncertain. The uncertainties in the representation of aerosol interactions in climate models makes it problematic to use model projections to guide energy policy. The objective of our program is to reduce the uncertainties in the aerosol radiative forcing in the two areas highlighted in the ASR Science and Program Plan. That is, (1) addressing the direct effect by correlating particle chemistry and morphology with particle optical properties (i.e. absorption, scattering, extinction), and (2) addressing the indirect effect by correlating particle hygroscopicity and CCN activity with particle size, chemistry, and morphology. In this connection we are systematically studying particle formation, oxidation, and the effects of particle coating. The work is specifically focused on carbonaceous particles where the uncertainties in the climate relevant properties are the highest. The ongoing work consists of laboratory experiments and related instrument inter-comparison studies both coordinated with field and modeling studies, with the aim of providing reliable data to represent aerosol processes in climate models. The work is performed in the aerosol laboratory at Boston College. At the center of our laboratory setup are two main sources for the production of aerosol particles: (a) two well-characterized source of soot particles and (b) a flow reactor for controlled OH and/or O3 oxidation of relevant gas phase species to produce well-characterized SOA particles. After formation, the aerosol particles are subjected to physical and chemical processes that simulate aerosol growth and aging. A suite of instruments in our laboratory is used to characterize the physical and chemical properties of aerosol particles before and after processing. The Time of Flight Aerosol Mass Spectrometer (ToF-AMS) together with a Scanning Mobility Particle Sizer (SMPS) measures particle mass, volume, density, composition (including black carbon content), dynamic shape factor, and fractal dimension. The-ToF-AMS was developed at ARI with Boston College participation. About 120 AMS instruments are now in service (including 5 built for DOE laboratories) performing field and laboratory studies world-wide. Other major instruments include a thermal denuder, two Differential Mobility Analyzers (DMA), a Cloud Condensation Nuclei Counter (CCN), a Thermal desorption Aerosol GC/MS (TAG) and the new Soot Particle Aerosol Mass Spectrometer (SP-AMS). Optical instrumentation required for the studies have been brought to our laboratory as part of ongoing and planned collaborative projects with colleagues from DOE, NOAA and university laboratories. Optical instruments that will be utilized include a Photoacoustic Spectrometer (PAS), a Cavity Ring Down Aerosol Extinction Spectrometer (CRD-AES), a Photo Thermal Interferometer (PTI), a new 7-wavelength Aethalometer and a Cavity Attenuated Phase Shift Extinction Monitor (CAPS). These instruments are providing aerosol absorption, extinction and scattering coefficients at a range of atmospherically relevant wavelengths. During the past two years our work has continued along the lines of our original proposal. We report on 12 completed and/or continuing projects conducted during the period 08/14 to 0814/2015. These projects are described in ...
Book Synopsis Carbonaceous Aerosol by : András Gelencsér
Download or read book Carbonaceous Aerosol written by András Gelencsér and published by Springer Science & Business Media. This book was released on 2007-09-28 with total page 357 pages. Available in PDF, EPUB and Kindle. Book excerpt: The concept of carbonaceous aerosol has only recently emerged from atmospheric pollution studies; even standard nomenclature and terminology are still unsettled. This monograph is the first to offer comprehensive coverage of the nature and atmospheric role of carbonaceous aerosol particles. Atmospheric chemists, physicists, meteorologists, and modellers will find this a thought-inspiring and sometimes provocative overview of all global phenomena affected by or related to carbonaceous aerosol.
Book Synopsis Particulate Carbon by : George T. Wolff
Download or read book Particulate Carbon written by George T. Wolff and published by Springer Science & Business Media. This book was released on 2012-12-06 with total page 405 pages. Available in PDF, EPUB and Kindle. Book excerpt: This book contains the papers and discussions from the symposium, "PARTICU LATE CARBON: Atmospheric Life Cycle," held at the General Motors Research Laboratories on October 13-14, 1980. This symposium, which focused on atmospheric particulate elemental carbon, or soot, was the twenty-fifth in this series sponsored by the General Motors Research Laboratories. The present symposium volume contains discussions of the following aspects of particulate elemental carbon (EC): the atmos pheric life cycle of EC including sources, sinks, and transport processes, the role of EC in atmospheric chemistry and optics, the possible role of EC in altering climate, and measurement techniques as well as ambient concentrations in urban, rural, and remote areas. Previous symposia have covered a wide range of scientific and engineering subjects. Topics are selected because they are new or represent rapidly changing fields and are of significant technical importance. It is ironic that the study of particulate elemental carbon or soot should meet the above criteria for selection because soot, especially from coal and wood combustion, has been a recognized air pollutant for centuries. However, since the 1950s, when intense efforts to study air pollution were initiated, to until a few years ago, the role of elemental carbon in the atmosphere was largely ignored. The major reason for this was the lack of a suitable measurement technique.
Book Synopsis Laboratory Experiments and Instrument Development for the Study of Atmospheric Aerosols by :
Download or read book Laboratory Experiments and Instrument Development for the Study of Atmospheric Aerosols written by and published by . This book was released on 2011 with total page pages. Available in PDF, EPUB and Kindle. Book excerpt: Soot particles are generated by incomplete combustion of fossil and biomass fuels. Through direct effects clear air aerosols containing black carbon (BC) such as soot aerosols, absorb incoming light heating the atmosphere, while most other aerosols scatter light and produce cooling. Even though BC represents only 1-2% of the total annual emissions of particulate mass to the atmosphere, it has been estimated that the direct radiative effect of BC is the second-most important contributor to global warming after absorption by CO2. Ongoing studies continue to underscore the climate forcing importance of black carbon. However, estimates of the radiative effects of black carbon on climate remain highly uncertain due to the complexity of particles containing black carbon. Quantitative measurement of BC is challenging because BC often occurs in highly non-spherical soot particles of complex morphology. Freshly emitted soot particles are typically fractal hydrophobic aggregates. The aggregates consist of black carbon spherules with diameters typically in the range of about 15-40 nm, and they are usually coated by adsorbed polyaromatic hydrocarbons (PAHs) produced during combustion. Diesel-generated soot particles are often emitted with an organic coating composed primarily of lubricating oil and unburned fuel, as well as well as PAH compounds. Sulfuric acid has also been detected in diesel and aircraft-emitted soot particles. In the course of aging, these particle coatings may be substantially altered by chemical reactions and/or the deposition of other materials. Such processes transform the optical and CCN properties of the soot aerosols in ways that are not yet well understood. Our work over the past seven years consisted of laboratory research, instrument development and characterization, and field studies with the central focus of improving our understanding of the black carbon aerosol climate impacts. During the sixth year as well as during this seventh year (no-cost extension period) of our grant, we extended our studies to perform experiments on the controlled production and characterization of secondary organic aerosol.
Book Synopsis The Implementation and Evaluation of a Black Carbon Aerosol Sampler Used on an Unmanned Aircraft During the Prescribed Fire Experiment RxCADRE by : Tara L. Craft
Download or read book The Implementation and Evaluation of a Black Carbon Aerosol Sampler Used on an Unmanned Aircraft During the Prescribed Fire Experiment RxCADRE written by Tara L. Craft and published by . This book was released on 2014 with total page 158 pages. Available in PDF, EPUB and Kindle. Book excerpt: Black carbon (BC) aerosols impact the earth's climate by absorbing solar radiation in the atmosphere and depositing on ice surfaces and lowering the albedo of those surfaces. Black carbon aerosols have been widely studied; however, using small unmanned aircraft systems (UAS) for the airborne study of the vertical and horizontal concentrations of BC is an emerging field. Using UAS to study BC poses some challenges due to size and weight restrictions of the aircraft, as well as issues that arise when adapting ground based instrumentation for use on different aircraft. University of Alaska Fairbanks researchers successfully integrated and flew a microAeth AE-51 on a Boeing ScanEagle to measure the concentration of BC and other absorbing and scattering particles in the smoke plume from a prescribed fire experiment, RxCADRE, conducted at Eglin AFB, FL, during October and November 2012. The ScanEaglemounted microAeth successfully collected black carbon aerosols in the smoke plume. The optical particle sizing and mass loadings from an optical particle counter disagreed with the results from the microAeth, which measures absorbing aerosols. The microAeth was tested in the laboratory-using two optical particle sizers to verify the sizes and concentrations of laboratory-generated aerosols entering the instrument and determine the capabilities and limits of the instrument. The optical particle counters were used in other applications as well showing the versatility of the instruments in extreme conditions.
Book Synopsis Aerosols in Atmospheric Chemistry by : Yue Zhang
Download or read book Aerosols in Atmospheric Chemistry written by Yue Zhang and published by American Chemical Society. This book was released on 2022-04-01 with total page 176 pages. Available in PDF, EPUB and Kindle. Book excerpt: The uncertainties in the aerosol effects on radiative forcing limit our knowledge of climate change, presenting us with an important research challenge. Aerosols in Atmospheric Chemistry introduces basic concepts about the characterization, formation, and impacts of ambient aerosol particles as an introduction to graduate students new to the field. Each chapter also provides an up-to-date synopsis of the latest knowledge of aerosol particles in atmospheric chemistry.
Book Synopsis Analysis of Atmospheric Aerosol Processes Using Single Particle Mass Spectrometry by : Jeffrey Robert Whiteaker
Download or read book Analysis of Atmospheric Aerosol Processes Using Single Particle Mass Spectrometry written by Jeffrey Robert Whiteaker and published by . This book was released on 2002 with total page 644 pages. Available in PDF, EPUB and Kindle. Book excerpt:
Book Synopsis Climate Implications of Carbonaceous Aerosols by :
Download or read book Climate Implications of Carbonaceous Aerosols written by and published by . This book was released on 2010 with total page pages. Available in PDF, EPUB and Kindle. Book excerpt: Recently, attention has been drawn towards black carbon aerosols as a likely short-term climate warming mitigation candidate. However the global and regional impacts of the direct, cloud-indirect and semi-direct forcing effects are highly uncertain, due to the complex nature of aerosol evolution and its climate interactions. Black carbon is directly released as particle into the atmosphere, but then interacts with other gases and particles through condensation and coagulation processes leading to further aerosol growth, aging and internal mixing. A detailed aerosol microphysical scheme, MATRIX, embedded within the global GISS modelE includes the above processes that determine the lifecycle and climate impact of aerosols. This study presents a quantitative assessment of the impact of microphysical processes involving black carbon, such as emission size distributions and optical properties on aerosol cloud activation and radiative forcing. Our best estimate for net direct and indirect aerosol radiative forcing change is -0.56 W/m2 between 1750 and 2000. However, the direct and indirect aerosol effects are very sensitive to the black and organic carbon size distribution and consequential mixing state. The net radiative forcing change can vary between -0.32 to -0.75 W/m2 depending on these carbonaceous particle properties. Assuming that sulfates, nitrates and secondary organics form a coating shell around a black carbon core, rather than forming a uniformly mixed particles, changes the overall net radiative forcing from a negative to a positive number. Black carbon mitigation scenarios showed generally a benefit when mainly black carbon sources such as diesel emissions are reduced, reducing organic and black carbon sources such as bio-fuels, does not lead to reduced warming.
Author :Panel on Aerosol Radiative Forcing and Climate Change Publisher :National Academies Press ISBN 13 :0309588871 Total Pages :180 pages Book Rating :4.3/5 (95 download)
Book Synopsis A Plan for a Research Program on Aerosol Radiative Forcing and Climate Change by : Panel on Aerosol Radiative Forcing and Climate Change
Download or read book A Plan for a Research Program on Aerosol Radiative Forcing and Climate Change written by Panel on Aerosol Radiative Forcing and Climate Change and published by National Academies Press. This book was released on 1996-05-01 with total page 180 pages. Available in PDF, EPUB and Kindle. Book excerpt: This book recommends the initiation of an "integrated" research program to study the role of aerosols in the predicted global climate change. Current understanding suggest that, even now, aerosols, primarily from anthropogenic sources, may be reducing the rate of warming caused by greenhouse gas emissions. In addition to specific research recommendations, this book forcefully argues for two kinds of research program integration: integration of the individual laboratory, field, and theoretical research activities and an integrated management structure that involves all of the concerned federal agencies.
Download or read book Aerosol Science written by Ian Colbeck and published by John Wiley & Sons. This book was released on 2014-02-03 with total page 522 pages. Available in PDF, EPUB and Kindle. Book excerpt: AEROSOL SCIENCE TECHNOLOGY AND APPLICATIONS Aerosols influence many areas of our daily life. They are at the core of environmental problems such as global warming, photochemical smog and poor air quality. They can also have diverse effects on human health, where exposure occurs in both outdoor and indoor environments. However, aerosols can have beneficial effects too; the delivery of drugs to the lungs, the delivery of fuels for combustion and the production of nanomaterials all rely on aerosols. Advances in particle measurement technologies have made it possible to take advantage of rapid changes in both particle size and concentration. Likewise, aerosols can now be produced in a controlled fashion. Reviewing many technological applications together with the current scientific status of aerosol modelling and measurements, this book includes: Satellite aerosol remote sensing The effects of aerosols on climate change Air pollution and health Pharmaceutical aerosols and pulmonary drug delivery Bioaerosols and hospital infections Particle emissions from vehicles The safety of emerging nanomaterials Radioactive aerosols: tracers of atmospheric processes With the importance of this topic brought to the public's attention after the eruption of the Icelandic volcano Eyjafjallajökull, this book provides a timely, concise and accessible overview of the many facets of aerosol science.
Book Synopsis Carbonaceous Aerosols and Radiative Effects Study (CARES), G1-aircraft, Sedlacek Sp2 by :
Download or read book Carbonaceous Aerosols and Radiative Effects Study (CARES), G1-aircraft, Sedlacek Sp2 written by and published by . This book was released on 2011 with total page pages. Available in PDF, EPUB and Kindle. Book excerpt: The primary objective of the Carbonaceous Aerosol and Radiative Effects Study (CARES) in 2010 was to investigate the evolution of carbonaceous aerosols of different types and their optical and hygroscopic properties in central California, with a focus on the Sacramento urban plume.
Book Synopsis Recent Advances in Aerosol Research by : C. N. Davies
Download or read book Recent Advances in Aerosol Research written by C. N. Davies and published by Elsevier. This book was released on 2013-10-22 with total page 91 pages. Available in PDF, EPUB and Kindle. Book excerpt: Recent Advances in Aerosol Research: A Bibliographical Review presents a bibliographic review of advances in aerosol research covering the period from the beginning of 1957 to the end of 1962. Topics covered include chemical reactions, combustion, coagulation and diffusion, and adhesion of particles. References on filtration, evaporation and condensation, nucleation and growth, and laminar flow and impingement are also included. This volume is comprised of 19 chapters and begins by citing research on acoustic, ultrasonic, and shock wave effects, along with adhesion of particles, chemical reactions, combustion, coagulation and diffusion, and filtration. The following chapters deal with evaporation and condensation, nucleation and growth, laminar flow and impingement, generators, photophoresis, and the optics of aerosols. Other chapters focus on radioactivity, sampling instruments, sedimentation and fluid resistance, thermophoresis, and diffusiophoresis. The last chapter highlights turbulent flow and deposition of aerosols. This monograph will be a valuable resource for researchers and practitioners interested in aerosols.
Book Synopsis Models for the Aerosols of the Lower Atmosphere and the Effects of Humidity Variations on Their Optical Properties by : Eric P. Shettle
Download or read book Models for the Aerosols of the Lower Atmosphere and the Effects of Humidity Variations on Their Optical Properties written by Eric P. Shettle and published by . This book was released on 1979 with total page 100 pages. Available in PDF, EPUB and Kindle. Book excerpt: Aerosol models have been developed for the lower atmosphere. These models are representative of conditions found in rural, urban, and maritime air masses. The changes in the aerosol properties with variations in the relative humidity are discussed. To describe the aerosol optical properties in the extreme of 100 percent relative humidity, several fog models are presented. For each model the coefficients for extinction, scattering, and absorption, the angular scattering distribution, and other optical parameters have been computed for wavelengths between 0.2 and 40 microns. These aerosol models are presented together with a review of their experimental basis. The optical properties of these models are discussed and some comparisons of the model with experimental measurements are presented.
Book Synopsis Investigation of Optical Properties of Size-selected Black Carbon Under Controlled Laboratory Conditions by : Ziying Lei
Download or read book Investigation of Optical Properties of Size-selected Black Carbon Under Controlled Laboratory Conditions written by Ziying Lei and published by . This book was released on 2016 with total page 80 pages. Available in PDF, EPUB and Kindle. Book excerpt: Air pollution, one of the most concerning and widespread environmental issues has grown in importance in the world. The carbonaceous aerosols significantly contribute to air pollution, which not only causes public health concern, but also impacts climate change. The aerosol particles have properties to absorb or scatter solar radiation and thermal radiation; therefore, they play an important role in climate change. In order to improve the understanding and control the aerosol particles, it is crucial to study aerosol size distribution and chemical compounds. Black carbon is the strongest radiative absorber suspends in the atmosphere, and can have great influence on climate change. This study investigates the size-selected black carbon optical properties under laboratory conditions with varied relative humidity referred to “dry”, “humid”, and “wet” respectively. The single scattering albedo that measures the relative amount of aerosol light extinction due to scattering, and the absorption enhancement due to lensing effect are measured in this study, and compared with the modeling results based on Mie theory, which is used to predict the absorption and scattering of light by a spherical particle. The results show that the single scattering albedo under the dry, humid, and wet conditions are similar, while the single scattering albedo for black carbon particles that have undergone heating to 160 oC is slightly greater than other three conditions. In general, with respect to particle size, single scattering albedo increases with smaller particle size and then levels off at larger size diameters. In addition, the absorption enhancement for black carbon particles is estimated in this study, and it ranges from 1 to 2.5. The values based on observations generally follow the predicted trend from Mie theory. Comparing the observed and modeled values suggests that 25%-50% of the total particle diameter is attributable to coating material. Dry black carbon particles do not have high absorption enhancement because they likely have no or thin coating materials. However, the absorption enhancement for humid particles and wet particles are higher than the dry particles, likely due to an enhanced lensing effect due to water uptake by the black carbon particles. Future study will focus on improving the understanding of black carbon optical properties and accuracy of experimental results. Further research is recommended to focus on ranges of BC particles with the diameters smaller than 100 nm and larger than 650 nm, which are not included in this study and constrain the particle charge units.
Download or read book Aerosols written by Pratim Biswas and published by Walter de Gruyter GmbH & Co KG. This book was released on 2022-07-18 with total page 224 pages. Available in PDF, EPUB and Kindle. Book excerpt: Aerosol science and engineering is a vibrant field of particle technology and chemical reaction engineering. The book presents a timely account of this interdisciplinary topic and its various application areas. It will be of interest to scientists or engineers active in aerosol physics, aerosol or colloid chemistry, atmospheric processes, and chemical, mechanical, environmental and/or materials engineering.
Book Synopsis Topics in Current Aerosol Research by : G. M. Hidy
Download or read book Topics in Current Aerosol Research written by G. M. Hidy and published by Elsevier. This book was released on 2013-10-22 with total page 393 pages. Available in PDF, EPUB and Kindle. Book excerpt: Topics in Current Aerosol Research, Part 2 contains some selected articles in the field of aerosol study. The chosen topics deal extensively with the theory of diffusiophoresis and thermophoresis. Also covered in the book is the mathematical treatment of integrodifferential equations originating from the theory of aerosol coagulation. The book is the third volume of the series entitled International Reviews in Aerosol Physics and Chemistry. The text offers significant understanding of the methods employed to develop a theory for thermophoretic and diffusiophoretic forces acting on spheres in the range from free molecules to continuum behavior. It explores the mathematical solution for the kinetic model of the coagulation equation. Another topic of interest is the means to estimate size dispersal function for clouds of particles undergoing collision. The text can be a useful tool for practicing scientists and graduate students in physics, meteorology, geophysics, physical chemistry, environmental science, medicine, chemical engineering, and aerospace engineering.
