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Download or read book Active Sites and Structure-Activity Relationship of Copper-Based Catalysts for Carbon Dioxide Hydrogenation to Methanol written by and published by . This book was released on 2012 with total page pages. Available in PDF, EPUB and Kindle. Book excerpt:
Author : Jerzy Skrzypek
Publisher :
ISBN 13 :
Total Pages : 174 pages
Book Rating : 4.F/5 ( download)
Download or read book Methanol Synthesis written by Jerzy Skrzypek and published by . This book was released on 1994 with total page 174 pages. Available in PDF, EPUB and Kindle. Book excerpt:
Author : Xiao Jiang
Publisher :
ISBN 13 :
Total Pages : pages
Book Rating : 4.:/5 (943 download)
Download or read book Palladium-Copper Bimetallic Catalysts for Selective Carbon Dioxide Hydrogenation to Methanol written by Xiao Jiang and published by . This book was released on 2015 with total page pages. Available in PDF, EPUB and Kindle. Book excerpt: Catalytic CO2 hydrogenation for synthesis of methanol has attracted significant attention recently as a way of recycling carbon dioxide as a resource. In the past decades, most prior works focused on Cu-based and supported Pd-based catalysts to hydrogenate CO2 to CH3OH. Cu and Pd were proposed to have different affinities towards the adsorption of CO2 and H2, respectively. However, little attention has been paid to the effect of Pd-Cu bimetallic catalysts on the methanol synthesis from CO2 hydrogenation. Thus, this work aims at studying the effect of combining Pd and Cu on the activity and selectivity of methanol synthesis via CO2 hydrogenation and developing a fundamental understanding on composition-structure-activity relationship. The Pd-Cu bimetallic catalysts with various compositions were prepared and examined in CO2 hydrogenation at relatively mild reaction conditions (523 K and 4.1 MPa).A strong synergistic effect was observed over Pd--Cu bimetallic catalysts supported on silica at specific compositions as evidenced from the superior methanol formation rate and selectivity in comparison to monometallic catalysts, and the optimal Pd/(Pd+Cu) atomic ratios lied in the range of 0.25-0.34. The methanol formation rate over Pd(8.7)-Cu(10)/SiO2 was almost three times higher than the simple sum of those over monometallic Cu and Pd catalysts. To investigate the composition-structure-activity relationship, the Pd-Cu bimetallic catalysts were characterized by X-ray diffraction (XRD), transmission electron microscopy (TEM), scanning transmission electron microscopy coupled with energy dispersive X-ray spectroscopy (STEM/EDS), X-ray photoelectron spectroscopy (XPS), hydrogen temperature-programmed reduction (H2-TPR), and temperature-programmed desorption (H2-, CO2-, & CO-TPD). Detailed characterization results demonstrated the importance of two well-dispersed Pd--Cu alloy particles (PdCu3 and PdCu) for the observed methanol promotion over Pd--Cu bimetallic catalysts. DRIFTS spectra revealed that the incorporation of Pd and Cu greatly improved the formation of formate and CO species during the CO2 hydrogenation. CO-TPD profiles confirmed the existence of three forms of chemisorbed CO species, and the bonding strength increased in the following order: COL (linear)
Author : Martin Bertau
Publisher : Springer Science & Business Media
ISBN 13 : 3642397093
Total Pages : 699 pages
Book Rating : 4.6/5 (423 download)
Download or read book Methanol: The Basic Chemical and Energy Feedstock of the Future written by Martin Bertau and published by Springer Science & Business Media. This book was released on 2014-02-18 with total page 699 pages. Available in PDF, EPUB and Kindle. Book excerpt: Methanol - The Chemical and Energy Feedstock of the Future offers a visionary yet unbiased view of methanol technology. Based on the groundbreaking 1986 publication "Methanol" by Friedrich Asinger, this book includes contributions by more than 40 experts from industry and academia. The authors and editors provide a comprehensive exposition of methanol chemistry and technology which is useful for a wide variety of scientists working in chemistry and energy related industries as well as academic researchers and even decision-makers and organisations concerned with the future of chemical and energy feedstocks.
Author : Moises Romolos Cesario
Publisher : Elsevier
ISBN 13 : 0323856322
Total Pages : 554 pages
Book Rating : 4.3/5 (238 download)
Download or read book Heterogeneous Catalysis written by Moises Romolos Cesario and published by Elsevier. This book was released on 2022-04-27 with total page 554 pages. Available in PDF, EPUB and Kindle. Book excerpt: Heterogeneous Catalysis: Materials and Applications focuses on heterogeneous catalysis applied to the elimination of atmospheric pollutants as an alternative solution for producing clean energy and the valorization of chemical products. The book helps users understand the properties of catalytic materials and catalysis phenomena governing electrocatalytic/catalytic reactions, and – more specifically – the study of surface and interface chemistry. By clustering knowledge in these fields, the book makes information available to both the academic and industrial communities. Further, it shows how heterogeneous catalysis applications can be used to solve environmental problems and convert energy through electrocatalytic reactions and chemical valorization. Sections cover nanomaterials for heterogeneous catalysis, heterogeneous catalysis mechanisms, SOX adsorption, greenhouse gases conversion, reforming reactions for hydrogen production, valorization of hydrogen energy, energy conversion and biomass valorization. Addresses topics of increasing interest to society such as the valorization of biomass, the use of polluting gases to produce value-added products, and the optimization of catalytic materials for water splitting, fuel cells, and other devices Discusses pollutant adsorption by industrial fume desulphurization processes Helps improve processes for obtaining chemicals using nonconventional technologies
Author : Annemie Bogaerts
Publisher : MDPI
ISBN 13 : 3038977500
Total Pages : 248 pages
Book Rating : 4.0/5 (389 download)
Download or read book Plasma Catalysis written by Annemie Bogaerts and published by MDPI. This book was released on 2019-04-02 with total page 248 pages. Available in PDF, EPUB and Kindle. Book excerpt: Plasma catalysis is gaining increasing interest for various gas conversion applications, such as CO2 conversion into value-added chemicals and fuels, N2 fixation for the synthesis of NH3 or NOx, methane conversion into higher hydrocarbons or oxygenates. It is also widely used for air pollution control (e.g., VOC remediation). Plasma catalysis allows thermodynamically difficult reactions to proceed at ambient pressure and temperature, due to activation of the gas molecules by energetic electrons created in the plasma. However, plasma is very reactive but not selective, and thus a catalyst is needed to improve the selectivity. In spite of the growing interest in plasma catalysis, the underlying mechanisms of the (possible) synergy between plasma and catalyst are not yet fully understood. Indeed, plasma catalysis is quite complicated, as the plasma will affect the catalyst and vice versa. Moreover, due to the reactive plasma environment, the most suitable catalysts will probably be different from thermal catalysts. More research is needed to better understand the plasma–catalyst interactions, in order to further improve the applications.
Author : Jean-Marie Basset
Publisher : Springer Science & Business Media
ISBN 13 : 9400929714
Total Pages : 340 pages
Book Rating : 4.4/5 (9 download)
Download or read book Surface Organometallic Chemistry: Molecular Approaches to Surface Catalysis written by Jean-Marie Basset and published by Springer Science & Business Media. This book was released on 2012-12-06 with total page 340 pages. Available in PDF, EPUB and Kindle. Book excerpt: Surface organometallic chemistry is a new field bringing together researchers from organometallic, inorganic, and surface chemistry and catalysis. Topics ranging from reaction mechanisms to catalyst preparation are considered from a molecular basis, according to which the "active site" on a catalyst surface has a supra-molecular character. This. the first book on the subject, is the outcome of a NATO Workshop held in Le Rouret. France, in May. 1986. It is our hope that the following chapters and the concluding summary of recommendations for research may help to provide a definition of surface organometallic chemistry. Besides catalysis. the central theme of the Workshop, four main topics are considered: 1) Reactions of organometallics with surfaces of metal oxides, metals. and zeolites; 2) Molecular models of surfaces, metal oxides, and metals; 3) Molecular approaches to the mechanisms of surface reactions; 4) Synthesis and modification of zeolites and related microporous solids. Most surface organometallic chemistry has been carried out on amorphous high-surf ace-area metal oxides such as silica. alumina. magnesia, and titania. The first chapter. contributed by KNOZINGER. gives a short summary of the structure and reactivity of metal oxide surfaces. Most of our understanding of these surfaces is based on acid base and redox chemistry; this chemistry has developed from X-ray and spectroscopic data, and much has been inferred from the structures and reactivities of adsorbed organic probe molecules. There are major opportunities for extending this understanding by use of well-defined (single crystal) oxide surfaces and organometallic probe molecules.
Author : Yuichiro Himeda
Publisher : John Wiley & Sons
ISBN 13 : 3527346635
Total Pages : 322 pages
Book Rating : 4.5/5 (273 download)
Download or read book CO2 Hydrogenation Catalysis written by Yuichiro Himeda and published by John Wiley & Sons. This book was released on 2021-06-28 with total page 322 pages. Available in PDF, EPUB and Kindle. Book excerpt: A guide to the effective catalysts and latest advances in CO2 conversion in chemicals and fuels Carbon dioxide hydrogenation is one of the most promising and economic techniques to utilize CO2 emissions to produce value-added chemicals. With contributions from an international team of experts on the topic, CO2 Hydrogenation Catalysis offers a comprehensive review of the most recent developments in the catalytic hydrogenation of carbon dioxide to formic acid/formate, methanol, methane, and C2+ products. The book explores the electroreduction of carbon dioxide and contains an overview on hydrogen production from formic acid and methanol. With a practical review of the advances and challenges in future CO2 hydrogenation research, the book provides an important guide for researchers in academia and industry working in the field of catalysis, organometallic chemistry, green and sustainable chemistry, as well as energy conversion and storage. This important book: Offers a unique review of effective catalysts and the latest advances in CO2 conversion Explores how to utilize CO2 emissions to produce value-added chemicals and fuels such as methanol, olefins, gasoline, aromatics Includes the latest research in homogeneous and heterogeneous catalysis as well as electrocatalysis Highlights advances and challenges for future investigation Written for chemists, catalytic chemists, electrochemists, chemists in industry, and chemical engineers, CO2 Hydrogenation Catalysis offers a comprehensive resource to understanding how CO2 emissions can create value-added chemicals.
Author : Martyn V. Twigg
Publisher : Routledge
ISBN 13 : 1351462326
Total Pages : 609 pages
Book Rating : 4.3/5 (514 download)
Download or read book Catalyst Handbook written by Martyn V. Twigg and published by Routledge. This book was released on 2018-12-19 with total page 609 pages. Available in PDF, EPUB and Kindle. Book excerpt: This book bridges the gap between theory and practice. It provides fundamental information on heterogeneous catalysis and the practicalities of the catalysts and processes used in producing ammonia, hydrogen and methanol via hydrocarbon steam reforming. It also covers the oxidation reactions in making formaldehyde from methanol, nitric acid from ammonia and sulphuric acid from sulphur dioxide. Designed for use in the chemical industry and by those in teaching, research and the study of industrial catalysts and catalytic processes. Students will also find this book extremely useful for obtaining practical information not available in more conventional textbooks.
Author : Gerhard Ertl
Publisher : John Wiley & Sons
ISBN 13 : 3527620680
Total Pages : 639 pages
Book Rating : 4.5/5 (276 download)
Download or read book Preparation of Solid Catalysts written by Gerhard Ertl and published by John Wiley & Sons. This book was released on 2008-08-29 with total page 639 pages. Available in PDF, EPUB and Kindle. Book excerpt: Solid catalysts play a fundamental role in all areas between basic research and industrial applications. This book offers a large amount of information about the preparation of solid catalysts. All types of solid catalysts and all important aspects of their preparation are discussed. The highly topical contributions are written by leading experts in disciplines ranging from solid state, interface and solution chemistry to industrial engineering. The straightforward presentation of the material and the comprehensive coverage make this book an essential and indispensible tool for every scientist and engineer working with solid catalysts.
Author : Vivek Polshettiwar
Publisher : John Wiley & Sons
ISBN 13 : 1118609808
Total Pages : 670 pages
Book Rating : 4.1/5 (186 download)
Download or read book Nanocatalysis written by Vivek Polshettiwar and published by John Wiley & Sons. This book was released on 2013-09-06 with total page 670 pages. Available in PDF, EPUB and Kindle. Book excerpt: Exhibiting both homogeneous and heterogeneous catalytic properties, nanocatalysts allow for rapid and selective chemical transformations, with the benefits of excellent product yield and ease of catalyst separation and recovery. This book reviews the catalytic performance and the synthesis and characterization of nanocatalysts, examining the current state of the art and pointing the way towards new avenues of research. Moreover, the authors discuss new and emerging applications of nanocatalysts and nanocatalysis, from pharmaceuticals to fine chemicals to renewable energy to biotransformations. Nanocatalysis features contributions from leading research groups around the world. These contributions reflect a thorough review of the current literature as well as the authors’ first-hand experience designing and synthesizing nanocatalysts and developing new applications for them. The book’s nineteen chapters offer a broad perspective, covering: Nanocatalysis for carbon-carbon and carbon-heteroatom coupling reactions Nanocatalysis for various organic transformations in fine chemical synthesis Nanocatalysis for oxidation, hydrogenation, and other related reactions Nanomaterial-based photocatalysis and biocatalysis Nanocatalysts to produce non-conventional energy such as hydrogen and biofuels Nanocatalysts and nano-biocatalysts in the chemical industry Readers will also learn about the latest spectroscopic and microscopy tools used in advanced characterization methods that shed new light on nanocatalysts and nanocatalysis. Moreover, the authors offer expert advice to help readers develop strategies to improve catalytic performance. Summarizing and reviewing all the most important advances in nanocatalysis over the last two decades, this book explains the many advantages of nanocatalysts over conventional homogeneous and heterogeneous catalysts, providing the information and guidance needed for designing green, sustainable catalytic processes.
Author : J. Isaac
Publisher :
ISBN 13 :
Total Pages : pages
Book Rating : 4.:/5 (643 download)
Download or read book Structure/activity Relationship of Cu/ZnO/Al203 Methanol Synthesis Catalysts written by J. Isaac and published by . This book was released on 1997 with total page pages. Available in PDF, EPUB and Kindle. Book excerpt:
Author : National Academies of Sciences, Engineering, and Medicine
Publisher : National Academies Press
ISBN 13 : 0309483360
Total Pages : 257 pages
Book Rating : 4.3/5 (94 download)
Download or read book Gaseous Carbon Waste Streams Utilization written by National Academies of Sciences, Engineering, and Medicine and published by National Academies Press. This book was released on 2019-02-22 with total page 257 pages. Available in PDF, EPUB and Kindle. Book excerpt: In the quest to mitigate the buildup of greenhouse gases in Earth's atmosphere, researchers and policymakers have increasingly turned their attention to techniques for capturing greenhouse gases such as carbon dioxide and methane, either from the locations where they are emitted or directly from the atmosphere. Once captured, these gases can be stored or put to use. While both carbon storage and carbon utilization have costs, utilization offers the opportunity to recover some of the cost and even generate economic value. While current carbon utilization projects operate at a relatively small scale, some estimates suggest the market for waste carbon-derived products could grow to hundreds of billions of dollars within a few decades, utilizing several thousand teragrams of waste carbon gases per year. Gaseous Carbon Waste Streams Utilization: Status and Research Needs assesses research and development needs relevant to understanding and improving the commercial viability of waste carbon utilization technologies and defines a research agenda to address key challenges. The report is intended to help inform decision making surrounding the development and deployment of waste carbon utilization technologies under a variety of circumstances, whether motivated by a goal to improve processes for making carbon-based products, to generate revenue, or to achieve environmental goals.
Author : Tomas Ramirez Reina
Publisher : John Wiley & Sons
ISBN 13 : 3527346392
Total Pages : 498 pages
Book Rating : 4.5/5 (273 download)
Download or read book Engineering Solutions for CO2 Conversion written by Tomas Ramirez Reina and published by John Wiley & Sons. This book was released on 2021-07-19 with total page 498 pages. Available in PDF, EPUB and Kindle. Book excerpt: A comprehensive guide that offers a review of the current technologies that tackle CO2 emissions The race to reduce CO2 emissions continues to be an urgent global challenge. "Engineering Solutions for CO2 Conversion" offers a thorough guide to the most current technologies designed to mitigate CO2 emissions ranging from CO2 capture to CO2 utilization approaches. With contributions from an international panel representing a wide range of expertise, this book contains a multidisciplinary toolkit that covers the myriad aspects of CO2 conversion strategies. Comprehensive in scope, it explores the chemical, physical, engineering and economical facets of CO2 conversion. "Engineering Solutions for CO2 Conversion" explores a broad range of topics including linking CFD and process simulations, membranes technologies for efficient CO2 capture-conversion, biogas sweetening technologies, plasma-assisted conversion of CO2, and much more. This important resource: * Addresses a pressing concern of global environmental damage, caused by the greenhouse gases emissions from fossil fuels * Contains a review of the most current developments on the various aspects of CO2 capture and utilization strategies * Incldues information on chemical, physical, engineering and economical facets of CO2 capture and utilization * Offers in-depth insight into materials design, processing characterization, and computer modeling with respect to CO2 capture and conversion Written for catalytic chemists, electrochemists, process engineers, chemical engineers, chemists in industry, photochemists, environmental chemists, theoretical chemists, environmental officers, "Engineering Solutions for CO2 Conversion" provides the most current and expert information on the many aspects and challenges of CO2 conversion.
Author : George A. Olah
Publisher : John Wiley & Sons
ISBN 13 : 3527644636
Total Pages : 351 pages
Book Rating : 4.5/5 (276 download)
Download or read book Beyond Oil and Gas written by George A. Olah and published by John Wiley & Sons. This book was released on 2011-08-24 with total page 351 pages. Available in PDF, EPUB and Kindle. Book excerpt: The world is currently consuming about 85 million barrels of oil a day, and about two-thirds as much natural gas equivalent, both derived from non-renewable natural sources. In the foreseeable future, our energy needs will come from any available alternate source. Methanol is one such viable alternative, and also offers a convenient solution for efficient energy storage on a large scale. In this updated and enlarged edition, renowned chemists discuss in a clear and readily accessible manner the pros and cons of humankind's current main energy sources, while providing new ways to overcome obstacles. Following an introduction, the authors look at the interrelationship of fuels and energy, and at the extent of our non-renewable fossil fuels. They also discuss the hydrogen economy and its significant shortcomings. The main focus is on the conversion of CO2 from industrial as well as natural sources into liquid methanol and related DME, a diesel fuel substitute that can replace LNG and LPG. The book is rounded off with an optimistic look at future possibilities. A forward-looking and inspiring work that vividly illustrates potential solutions to our energy and environmental problems.
Author : José J. G. Moura
Publisher : Springer Nature
ISBN 13 : 3030583155
Total Pages : 507 pages
Book Rating : 4.0/5 (35 download)
Download or read book Enzymes for Solving Humankind's Problems written by José J. G. Moura and published by Springer Nature. This book was released on 2020-12-01 with total page 507 pages. Available in PDF, EPUB and Kindle. Book excerpt: This book presents specific key natural and artificial systems that are promising biocatalysts in the areas of health, agriculture, environment and energy. It provides a comprehensive account of the state of the art of these systems and outlines the significant progress made in the last decade using these systems to develop innovative, sustainable and environmentally friendly solutions. Chapters from expert contributors explore how natural enzymes and artificial systems tackle specific targets such as: climate change, carbon footprint and economy and carbon dioxide utilisation; nitrogen footprint and fixation and nitrous oxide mitigation; hydrogen production, fuel cells and energy from bacteria; biomass transformation and production of added-value compounds, as well as biosensors development. This book provides an important and inspiring account for the designing of new natural and artificial systems with enhanced properties, and it appeals not only to students and researchers working in the fields of energy, health, food and environment, but also to a wider audience of educated readers that are interested in these up-to-date and exciting subjects. Chapter “Carbon Dioxide Utilisation—The Formate Route” is available open access under a Creative Commons Attribution 4.0 International License via link.springer.com.
Author : David Lloyd Roberts
Publisher :
ISBN 13 :
Total Pages : 346 pages
Book Rating : 4.:/5 (319 download)
Download or read book Identification and Characterization of Active Sites and Stable Surface Intermediates on Copper-based Methanol Synthesis Catalysts by Temperature-programmed Desorption and FTIR Spectroscopy written by David Lloyd Roberts and published by . This book was released on 1987 with total page 346 pages. Available in PDF, EPUB and Kindle. Book excerpt:
